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Resurgence and advancement of photochemical hydrogen atom transfer processes in selective alkane functionalizations
The selective functionalization of alkanes has long been recognized as a prominent
challenge and an arduous task in organic synthesis. Hydrogen atom transfer (HAT) …
challenge and an arduous task in organic synthesis. Hydrogen atom transfer (HAT) …
Homogeneous functionalization of methane
One of the remaining “grand challenges” in chemistry is the development of a next
generation, less expensive, cleaner process that can allow the vast reserves of methane …
generation, less expensive, cleaner process that can allow the vast reserves of methane …
Selective functionalization of methane, ethane, and higher alkanes by cerium photocatalysis
With the recent soaring production of natural gas, the use of methane and other light
hydrocarbon feedstocks as starting materials in synthetic transformations is becoming …
hydrocarbon feedstocks as starting materials in synthetic transformations is becoming …
Chemical and reactive transport processes associated with hydraulic fracturing of unconventional oil/gas shales
Hydraulic fracturing of unconventional oil/gas shales has changed the energy landscape of
the US Recovery of hydrocarbons from tight, hydraulically fractured shales is a highly …
the US Recovery of hydrocarbons from tight, hydraulically fractured shales is a highly …
Beyond ferryl-mediated hydroxylation: 40 years of the rebound mechanism and C–H activation
Since our initial report in 1976, the oxygen rebound mechanism has become the consensus
mechanistic feature for an expanding variety of enzymatic C–H functionalization reactions …
mechanistic feature for an expanding variety of enzymatic C–H functionalization reactions …
Methane conversion into different hydrocarbons or oxygenates: current status and future perspectives in catalyst development and reactor operation
This Perspective highlights recent developments in methane conversion into different
hydrocarbons and oxygenates (methanol, its derivatives, and formaldehyde) with the …
hydrocarbons and oxygenates (methanol, its derivatives, and formaldehyde) with the …
Large-scale selective functionalization of alkanes
Great progress has been made in the past several decades concerning C–H bond
functionalization. But despite many significant advances, a commercially viable large-scale …
functionalization. But despite many significant advances, a commercially viable large-scale …
Partial oxidation of methane enabled by decatungstate photocatalysis coupled to free radical chemistry
The decatungstate anion,[W10O32] 4–or DT, is a useful photocatalyst for organic
transformations involving C–H functionalization. Herein, we leverage the unique photoredox …
transformations involving C–H functionalization. Herein, we leverage the unique photoredox …
Alkane C–H functionalization and oxidation with molecular oxygen
The application of environmentally benign, cheap, and economically viable oxidation
procedures is a key challenge of homogeneous, oxidative alkane functionalization. The …
procedures is a key challenge of homogeneous, oxidative alkane functionalization. The …
A metal-free, photocatalytic method for aerobic alkane iodination
Halogenation is an important alkane functionalization strategy, but O2 is widely considered
the most desirable terminal oxidant. Here, the aerobic iodination of alkanes, including …
the most desirable terminal oxidant. Here, the aerobic iodination of alkanes, including …