Materials data toward machine learning: advances and challenges

L Zhu, J Zhou, Z Sun - The Journal of Physical Chemistry Letters, 2022 - ACS Publications
Machine learning (ML) is believed to have enabled a paradigm shift in materials research,
and in practice, ML has demonstrated its power in speeding up the cost-efficient discovery of …

Ultrafast X-ray probes of elementary molecular events

D Keefer, SM Cavaletto, JR Rouxel… - Annual Review of …, 2023 - annualreviews.org
Elementary events that determine photochemical outcomes and molecular functionalities
happen on the femtosecond and subfemtosecond timescales. Among the most ubiquitous …

Terawatt-scale attosecond X-ray pulses from a cascaded superradiant free-electron laser

P Franz, S Li, T Driver, RR Robles, D Cesar, E Isele… - Nature …, 2024 - nature.com
Intense attosecond X-ray pulses are key for ultrafast nonlinear spectroscopy and diffractive
imaging. Here we demonstrate the generation of terawatt-scale isolated attosecond pulses …

Experimental demonstration of attosecond pump–probe spectroscopy with an X-ray free-electron laser

Z Guo, T Driver, S Beauvarlet, D Cesar, J Duris… - Nature …, 2024 - nature.com
Pump–probe experiments with subfemtosecond resolution are the key to understanding
electronic dynamics in quantum systems. Here we demonstrate the generation and control …

Compact realization of all-attosecond pump-probe spectroscopy

M Kretschmar, E Svirplys, M Volkov, T Witting… - Science …, 2024 - science.org
The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a
longstanding goal in ultrafast science. While first pioneering experiments demonstrated the …

Attosecond delays in X-ray molecular ionization

T Driver, M Mountney, J Wang, L Ortmann… - Nature, 2024 - nature.com
The photoelectric effect is not truly instantaneous but exhibits attosecond delays that can
reveal complex molecular dynamics,,,,,–. Sub-femtosecond-duration light pulses provide the …

Separation of photoionization and measurement-induced delays

M Han, JB Ji, CS Leung, K Ueda, HJ Wörner - Science Advances, 2024 - science.org
Photoionization of matter is one of the fastest electronic processes in nature. Experimental
measurements of photoionization dynamics have become possible through attosecond …

Observation of attosecond time delays in above-threshold ionization

W **e, Z Li, M Li, Y Liu, Y Liu, C Cao, K Guo, K Liu… - Physical Review Letters, 2024 - APS
Attosecond-scale temporal characterization of photoionization is essential in understanding
how light and matter interact on the most fundamental level. However, characterizing the …

Attosecond investigation of extreme-ultraviolet multi-photon multi-electron ionization

M Kretschmar, A Hadjipittas, B Major, J Tümmler, I Will… - Optica, 2022 - opg.optica.org
Multi-<? TeX 2pc 0pt?> electron<? TeX 4pc 0pt?> dynamics in atoms and molecules very
often occur on sub-to few-femtosecond time scales. The available intensities of extreme …

Time-resolved experiments on gas-phase atoms and molecules with XUV and X-ray free-electron lasers

D Rolles - Advances in Physics: X, 2023 - Taylor & Francis
Over the last 20 years, XUV and X-ray free-electron lasers have enabled a wide variety of
time-resolved experiments that have dramatically advanced our understanding of ultrafast …