Mild metal-catalyzed C–H activation: examples and concepts

T Gensch, MN Hopkinson, F Glorius… - Chemical Society …, 2016‏ - pubs.rsc.org
Organic reactions that involve the direct functionalization of non-activated C–H bonds
represent an attractive class of transformations which maximize atom-and step-economy …

C− H functionalisation for hydrogen isotope exchange

J Atzrodt, V Derdau, WJ Kerr… - Angewandte Chemie …, 2018‏ - Wiley Online Library
The various applications of hydrogen isotopes (deuterium, D, and tritium, T) in the physical
and life sciences demand a range of methods for their installation in an array of molecular …

Exploiting hexafluoroisopropanol (HFIP) in Lewis and Brønsted acid-catalyzed reactions

V Pozhydaiev, M Power, V Gandon, J Moran… - Chemical …, 2020‏ - pubs.rsc.org
Hexafluoroisopropanol (HFIP) is a solvent with unique properties that has recently gained
attention for promoting a wide range of challenging chemical reactions. It was initially …

Computational studies of carboxylate-assisted C–H activation and functionalization at group 8–10 transition metal centers

DL Davies, SA Macgregor, CL McMullin - Chemical reviews, 2017‏ - ACS Publications
Computational studies on carboxylate-assisted C–H activation and functionalization at
group 8–10 transition metal centers are reviewed. This Review is organized by metal and …

Lewis superacids: classifications, candidates, and applications

L Greb - Chemistry–A European Journal, 2018‏ - Wiley Online Library
Lewis acids play a major role in all areas of chemistry. For a long time, toxic, corrosive and
oxidizing SbF5 was considered as the strongest Lewis acid known. Lately, species …

Platinum-catalyzed C–H functionalization

JA Labinger - Chemical Reviews, 2017‏ - ACS Publications
Recent developments in C–H bond activation and functionalization by Pt complexes are
surveyed. Topics include the following: fundamental mechanistic investigations of C–H …

Palladium-catalyzed nondirected late-stage C–H deuteration of arenes

M Farizyan, A Mondal, S Mal, F Deufel… - Journal of the …, 2021‏ - ACS Publications
We describe a palladium-catalyzed nondirected late-stage deuteration of arenes. Key
aspects include the use of D2O as a convenient and easily available deuterium source and …

Deuteration and Tritiation of Pharmaceuticals by Non‐Directed Palladium‐Catalyzed C− H Activation in Heavy and Super‐Heavy Water

C Teja, S Kolb, P Colonna, J Grover… - Angewandte Chemie …, 2024‏ - Wiley Online Library
Deuterated and tritiated analogs of drugs are valuable compounds for pharmaceutical and
medicinal chemistry. In this work, we present a novel hydrogen isotope exchange reaction of …

New trends in oxidative functionalization of carbon–hydrogen bonds: A review

GB Shul'pin - Catalysts, 2016‏ - mdpi.com
This review describes new reactions catalyzed by recently discovered types of metal
complexes and catalytic systems (catalyst+ co-catalyst). Works of recent years (mainly 2010 …

The power of the proton: from superacidic media to superelectrophile catalysis

HFT Klare, M Oestreich - Journal of the American Chemical …, 2021‏ - ACS Publications
Superacidic media became famous in connection with carbocations. Yet not all reactive
intermediates can be generated, characterized, and eventually isolated from these Brønsted …