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A review of the alpha radiolysis of extractants for actinide lanthanide separation in spent nuclear fuel reprocessing
Y Wang, Y Wan, Y Cai, L Yuan, W Feng, N Liu - Radiochimica Acta, 2021 - degruyter.com
Radiation stability is one of the key properties to enable the efficient use of extractants in
spent nuclear fuel with high radioactivity. The last several decades have witnessed a rapid …
spent nuclear fuel with high radioactivity. The last several decades have witnessed a rapid …
Radiolysis of diamide phenanthroline extractant: exploring the mechanism of HNO3 enhancing the extraction and An/Ln separation performance after irradiation
Y Chen, P Zhang, X Yang, Q Guo, H Weng… - Separation and …, 2023 - Elsevier
The stability of organic extractant molecules against radiolysis is critical in the field of
actinides and lanthanides (An/Ln) separations. In order to evaluate the radiolytic effects on …
actinides and lanthanides (An/Ln) separations. In order to evaluate the radiolytic effects on …
Impact of lanthanide ion complexation and temperature on the chemical reactivity of N, N, N′, N′-tetraoctyl diglycolamide (TODGA) with the dodecane radical cation
The impact of trivalent lanthanide ion complexation and temperature on the chemical
reactivity of N, N, N′, N′-tetraoctyl diglycolamide (TODGA) with the n-dodecane radical …
reactivity of N, N, N′, N′-tetraoctyl diglycolamide (TODGA) with the n-dodecane radical …
Effect of f-element complexation on the radiolysis of 2-ethylhexylphosphonic acid mono-2-ethylhexyl ester (HEH [EHP])
A systematic study of the impact on the chemical reactivity of the oxidising n-dodecane
radical cation (RH˙+) with f-element complexed 2-ethylhexylphosphonic acid mono-2 …
radical cation (RH˙+) with f-element complexed 2-ethylhexylphosphonic acid mono-2 …
Influence of uranyl complexation on the reaction kinetics of the dodecane radical cation with used nuclear fuel extraction ligands (TBP, DEHBA, and DEHiBA)
Specialized extractant ligands–such as tri-butyl phosphate (TBP), N, N-di-(2-ethylhexyl)
butyramide (DEHBA), and N, N-di-2-ethylhexylisobutryamide (DEHiBA)–have been …
butyramide (DEHBA), and N, N-di-2-ethylhexylisobutryamide (DEHiBA)–have been …
Evaluation of the Arrhenius behavior of n-dodecane radical cation (RH˙+) reactivity with lanthanide ion-complexed N, N, N′, N′-tetraoctyl diglycolamide (TODGA)
Temperature-dependent rate constants for the reaction of the n-dodecane radical cation
(RH˙+) with trivalent lanthanide ion-complexed N, N, N′, N′-tetraoctyl diglycolamide …
(RH˙+) with trivalent lanthanide ion-complexed N, N, N′, N′-tetraoctyl diglycolamide …
Gamma radiolytic stability of the novel modified diglycolamide 2, 2′-oxybis (N, N-didecylpropanamide)(mTDDGA) for grouped actinide extraction
B Verlinden, K Van Hecke, A Wilden, M Hupert… - RSC …, 2022 - pubs.rsc.org
Reprocessing of spent nuclear fuel aims at improving resource efficiency and reducing its
radiotoxicity and heat production in the long term. The necessary separation of certain metal …
radiotoxicity and heat production in the long term. The necessary separation of certain metal …
Radiation-induced effects on the extraction properties of hexa-n-octylnitrilo-triacetamide (HONTA) complexes of americium and europium
T Toigawa, DR Peterman, DS Meeker… - Physical Chemistry …, 2021 - pubs.rsc.org
The candidate An (III)/Ln (III) separation ligand hexa-n-octylnitrilo-triacetamide (HONTA) was
irradiated under envisioned SELECT (Solvent Extraction from Liquid waste using Extractants …
irradiated under envisioned SELECT (Solvent Extraction from Liquid waste using Extractants …
Does addition of 1-octanol as a phase modifier provide radical scavenging radioprotection for N, N, N′, N′-tetraoctyldiglycolamide (TODGA)?
To mitigate third phase formation in next generation used nuclear fuel reprocessing
technologies, the addition of 1-octanol has been trialed. However, contradictory reports on …
technologies, the addition of 1-octanol has been trialed. However, contradictory reports on …
Experimental and theoretical insights into the influence of gamma irradiation degradation products of N, N, N′, N′-tetraoctyl diglycolamide on extraction efficiency …
Y Wan, Y Li, J Liu, Q Li, Y Cai, X Li, S Ding… - Journal of Molecular …, 2024 - Elsevier
Understanding the effect of radiation rays on N, N, N′, N′-tetraoctyl diglycolamide
(TODGA) based solvent extraction systems is an essential task for establishing and …
(TODGA) based solvent extraction systems is an essential task for establishing and …