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Water oxidation in photosystem II
Biological water oxidation, performed by a single enzyme, photosystem II, is a central
research topic not only in understanding the photosynthetic apparatus but also for the …
research topic not only in understanding the photosynthetic apparatus but also for the …
Current understanding of the mechanism of water oxidation in photosystem II and its relation to XFEL data
The investigation of water oxidation in photosynthesis has remained a central topic in
biochemical research for the last few decades due to the importance of this catalytic process …
biochemical research for the last few decades due to the importance of this catalytic process …
Untangling the sequence of events during the S2 → S3 transition in photosystem II and implications for the water oxidation mechanism
In oxygenic photosynthesis, light-driven oxidation of water to molecular oxygen is carried out
by the oxygen-evolving complex (OEC) in photosystem II (PS II). Recently, we reported the …
by the oxygen-evolving complex (OEC) in photosystem II (PS II). Recently, we reported the …
One of the Substrate Waters for O2 Formation in Photosystem II Is Provided by the Water-Splitting Mn4CaO5 Cluster's Ca2+ Ion
CJ Kim, RJ Debus - Biochemistry, 2019 - ACS Publications
During the catalytic step immediately prior to O–O bond formation in Photosystem II, a water
molecule deprotonates and moves next to the water-splitting Mn4CaO5 cluster's O5 oxo …
molecule deprotonates and moves next to the water-splitting Mn4CaO5 cluster's O5 oxo …
Mechanism of Oxygen Evolution and Mn4CaO5 Cluster Restoration in the Natural Water-Oxidizing Catalyst
Water oxidation occurring in the first steps of natural oxygenic photosynthesis is catalyzed by
the pigment/protein complex Photosystem II. This process takes place on the Mn4Ca cluster …
the pigment/protein complex Photosystem II. This process takes place on the Mn4Ca cluster …
Structural isomers of the S2 state in photosystem II: do they exist at room temperature and are they important for function?
In nature, an oxo‐bridged Mn4CaO5 cluster embedded in photosystem II (PSII), a
membrane‐bound multi‐subunit pigment protein complex, catalyzes the water oxidation …
membrane‐bound multi‐subunit pigment protein complex, catalyzes the water oxidation …
Mutation-induced shift of the photosystem II active site reveals insight into conserved water channels
Photosystem II (PSII) is the water-plastoquinone photo-oxidoreductase central to oxygenic
photosynthesis. PSII has been extensively studied for its ability to catalyze light-driven water …
photosynthesis. PSII has been extensively studied for its ability to catalyze light-driven water …
Alteration of the O2-Producing Mn4Ca Cluster in Photosystem II by the Mutation of a Metal Ligand
RJ Debus - Biochemistry, 2021 - ACS Publications
The O2-evolving Mn4Ca cluster in photosystem II (PSII) is arranged as a distorted Mn3Ca
cube that is linked to a fourth Mn ion (denoted as Mn4) by two oxo bridges. The Mn4 and Ca …
cube that is linked to a fourth Mn ion (denoted as Mn4) by two oxo bridges. The Mn4 and Ca …
Role of the O4 channel in photosynthetic water oxidation as revealed by Fourier transform infrared difference and time-resolved infrared analysis of the D1-S169A …
Photosynthetic water oxidation takes place at the Mn4CaO5 cluster in photosystem II.
Although the atomic structures of its intermediates called S states have recently been …
Although the atomic structures of its intermediates called S states have recently been …
D1-S169A substitution of photosystem II perturbs water oxidation
In photosystem II (PSII), photosynthetic water oxidation occurs at the tetramanganese–
calcium cluster that cycles through light-induced intermediates (S0–S4) to produce oxygen …
calcium cluster that cycles through light-induced intermediates (S0–S4) to produce oxygen …