Electrochemical reduction of carbon dioxide to multicarbon (C 2+) products: challenges and perspectives

B Chang, H Pang, F Raziq, S Wang… - Energy & …, 2023 - pubs.rsc.org
Electrocatalytic CO2 reduction has been developed as a promising and attractive strategy to
achieve carbon neutrality for sustainable chemical production. Among various reduction …

Co-catalytic metal–support interactions in single-atom electrocatalysts

L Gloag, SV Somerville, JJ Gooding… - Nature Reviews Materials, 2024 - nature.com
Single-atom catalysts (SACs) are advantageous because every active atom is exposed at
the surface, ensuring maximum utilization of catalytically active metals. To optimize the …

Iridium single atoms incorporated in Co3O4 efficiently catalyze the oxygen evolution in acidic conditions

Y Zhu, J Wang, T Koketsu, M Kroschel, JM Chen… - Nature …, 2022 - nature.com
Designing active and stable electrocatalysts with economic efficiency for acidic oxygen
evolution reaction is essential for develo** proton exchange membrane water …

Carbon nitride based materials: more than just a support for single-atom catalysis

GFSR Rocha, MAR da Silva, A Rogolino… - Chemical Society …, 2023 - pubs.rsc.org
Recently, the missing link between homogeneous and heterogeneous catalysis has been
found and it was named single-atom catalysis (SAC). However, the SAC field still faces …

Gas diffusion electrodes, reactor designs and key metrics of low-temperature CO2 electrolysers

D Wakerley, S Lamaison, J Wicks, A Clemens… - Nature Energy, 2022 - nature.com
CO2 emissions can be recycled via low-temperature CO2 electrolysis to generate products
such as carbon monoxide, ethanol, ethylene, acetic acid, formic acid and propanol. In recent …

Metal ions confined in periodic pores of MOFs to embed single‐metal atoms within hierarchically porous carbon nanoflowers for high‐performance electromagnetic …

X Zhang, B Li, J Xu, X Zhang, Y Shi… - Advanced Functional …, 2023 - Wiley Online Library
Nanocarbons with single‐metal atoms (M‐SAs) have displayed considerable potential in
various fields of application due to high free energy of M‐SAs and strong metal‐support …

Spatially and temporally understanding dynamic solid–electrolyte interfaces in carbon dioxide electroreduction

J Wang, HY Tan, MY Qi, JY Li, ZR Tang… - Chemical Society …, 2023 - pubs.rsc.org
The ubiquity of solid–liquid interfaces in nature and the significant role of their atomic-scale
structure in determining interfacial properties have led to intensive research. Particularly in …

Regulating reconstruction of oxide-derived Cu for electrochemical CO2 reduction toward n-propanol

C Long, X Liu, K Wan, Y Jiang, P An, C Yang, G Wu… - Science …, 2023 - science.org
Oxide-derived copper (OD-Cu) is the most efficient and likely practical electrocatalyst for
CO2 reduction toward multicarbon products. However, the inevitable but poorly understood …

Covalent organic frameworks towards photocatalytic applications: Design principles, achievements, and opportunities

S Liu, M Wang, Y He, Q Cheng, T Qian… - Coordination Chemistry …, 2023 - Elsevier
As a subclass of porous framework materials, covalent organic frameworks (COFs) feature
permanent porosity, long-range order, and rigid backbones, and offer an important material …

Single atoms meet metal–organic frameworks: collaborative efforts for efficient photocatalysis

H Liu, M Cheng, Y Liu, J Wang, G Zhang, L Li… - Energy & …, 2022 - pubs.rsc.org
Photocatalysts with metal single atoms (SAs) as active sites have attracted widespread
interest owing to their maximum atomic utilization efficiency, well-defined active centers and …