Quantum chemistry in the age of quantum computing

Y Cao, J Romero, JP Olson, M Degroote… - Chemical …, 2019 - ACS Publications
Practical challenges in simulating quantum systems on classical computers have been
widely recognized in the quantum physics and quantum chemistry communities over the …

Atomic orbital basis sets

F Jensen - Wiley Interdisciplinary Reviews: Computational …, 2013 - Wiley Online Library
Electronic structure methods for molecular systems rely heavily on using basis sets
composed of Gaussian functions for representing the molecular orbitals. A number of …

An Extensive Set of Accurate Fluoride Ion Affinities for p‐Block Element Lewis Acids and Basic Design Principles for Strong Fluoride Ion Acceptors

P Erdmann, J Leitner, J Schwarz, L Greb - ChemPhysChem, 2020 - Wiley Online Library
The computed fluoride ion affinity (FIA) is a valuable descriptor to assess the Lewis acidity of
a compound. Despite its widespread use, the varying accuracy of applied computational …

Elevating density functional theory to chemical accuracy for water simulations through a density-corrected many-body formalism

S Dasgupta, E Lambros, JP Perdew… - Nature communications, 2021 - nature.com
Density functional theory (DFT) has been extensively used to model the properties of water.
Albeit maintaining a good balance between accuracy and efficiency, no density functional …

Segmented contracted basis sets optimized for nuclear magnetic shielding

F Jensen - Journal of Chemical Theory and Computation, 2015 - ACS Publications
A family of segmented contracted basis sets is proposed, denoted pcSseg-n, which are
optimized for calculating nuclear magnetic shielding constants. For the elements H–Ar …

Unifying general and segmented contracted basis sets. Segmented polarization consistent basis sets

F Jensen - Journal of chemical theory and computation, 2014 - ACS Publications
We propose a method, denoted P-orthogonalization, for converting a general contracted
basis set to a computationally more efficient segmented contracted basis set, while inheriting …

How good is the density-corrected SCAN functional for neutral and ionic aqueous systems, and what is so right about the Hartree–Fock density?

S Dasgupta, C Shahi, P Bhetwal… - Journal of Chemical …, 2022 - ACS Publications
Density functional theory (DFT) is the most widely used electronic structure method, due to
its simplicity and cost effectiveness. The accuracy of a DFT calculation depends not only on …

Enzymatic synthesis of azide by a promiscuous N-nitrosylase

A Del Rio Flores, R Zhai, DW Kastner, K Seshadri… - Nature Chemistry, 2024 - nature.com
Azides are energy-rich compounds with diverse representation in a broad range of scientific
disciplines, including material science, synthetic chemistry, pharmaceutical science and …

Revisiting the Atomic Natural Orbital Approach for Basis Sets: Robust Systematic Basis Sets for Explicitly Correlated and Conventional Correlated ab initio Methods?

F Neese, EF Valeev - Journal of chemical theory and computation, 2011 - ACS Publications
The performance of several families of basis sets for correlated wave function calculations
on molecules is studied. The widely used correlation-consistent basis set family cc-pVXZ (n …

Evaluating transition metal barrier heights with the latest density functional theory exchange–correlation functionals: The MOBH35 benchmark database

MA Iron, T Janes - The Journal of Physical Chemistry A, 2019 - ACS Publications
A new database of transition metal reaction barrier heights (MOBH35) is presented.
Benchmark energies (forward and reverse barriers and reaction energy) are calculated …