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Unifying nonlinear response and incoherent mixing in action-2D electronic spectroscopy
Action-detection has expanded the scope and applicability of 2D electronic spectroscopy,
while posing new challenges for the unambiguous interpretation of spectral features. In this …
while posing new challenges for the unambiguous interpretation of spectral features. In this …
Nonlinear optical spectroscopy of molecular assemblies: What is gained and lost in action detection?
This study elucidates the information content that is extracted from action-2D electronic
spectroscopy (A-2DES) when the output intensity is not proportional to the number of …
spectroscopy (A-2DES) when the output intensity is not proportional to the number of …
Expanding the bandwidth of fluorescence-detected two-dimensional electronic spectroscopy using a broadband continuum probe pulse pair
We demonstrate fluorescence-detected two-dimensional electronic spectroscopy (F-2DES)
with a broadband, continuum probe pulse pair in the pump-probe geometry. The approach …
with a broadband, continuum probe pulse pair in the pump-probe geometry. The approach …
Photosynthetic energy transfer: Missing in action (detected spectroscopy)?
A Javed, J Lüttig, K Charvátová… - The Journal of …, 2024 - ACS Publications
In recent years, action-detected ultrafast spectroscopies have gained popularity offering
distinct advantages over their coherently detected counterparts, such as spatially resolved …
distinct advantages over their coherently detected counterparts, such as spatially resolved …
Photoelectrochemical Two-Dimensional Electronic Spectroscopy (PEC2DES) of Photosystem I: Charge Separation Dynamics Hidden in a Multichromophoric …
We present a nonlinear spectroelectrochemical technique to investigate photosynthetic
protein complexes. The PEC2DES setup combines photoelectrochemical detection (PEC) …
protein complexes. The PEC2DES setup combines photoelectrochemical detection (PEC) …
A spectrometer design that eliminates incoherent mixing signals in 2D action spectroscopies
Action spectroscopies use a readout created by the action of light on the molecules or
material rather than optical absorption. Ultrafast 2D photocurrent and 2D fluorescence …
material rather than optical absorption. Ultrafast 2D photocurrent and 2D fluorescence …
Uncovering transport mechanisms in perovskite materials and devices with recombination-induced action spectroscopies
Although valuable insights are derived from conventional spectroscopic approaches, the
understanding of a photovoltaic device's operation mechanisms can be limited in ex situ …
understanding of a photovoltaic device's operation mechanisms can be limited in ex situ …
Resolving nonlinear recombination dynamics in semiconductors via ultrafast excitation correlation spectroscopy: Photoluminescence versus photocurrent detection
We explore the application of excitation correlation spectroscopy to detect nonlinear
photophysical dynamics in two distinct semiconductor classes through time-integrated …
photophysical dynamics in two distinct semiconductor classes through time-integrated …
Two-Dimensional Spectroscopy of Open Quantum Systems: Nonequilibrium Green's Function Formulation
Two-dimensional spectroscopy is examined for open quantum systems featuring multiple
simultaneously measurable fluxes. Specifically, we explore a junction where optical …
simultaneously measurable fluxes. Specifically, we explore a junction where optical …
[HTML][HTML] Exciton–photocarrier interference in mixed lead-halide-perovskite nanocrystals
The use of semiconductor nanocrystals in scalable quantum technologies requires
characterization of the exciton coherence dynamics in an ensemble of electronically isolated …
characterization of the exciton coherence dynamics in an ensemble of electronically isolated …