The ITensor software library for tensor network calculations

M Fishman, S White, EM Stoudenmire - SciPost Physics Codebases, 2022 - scipost.org
ITensor is a system for programming tensor network calculations with an interface modeled
on tensor diagram notation, which allows users to focus on the connectivity of a tensor …

The chromium dimer: closing a chapter of quantum chemistry

HR Larsson, H Zhai, CJ Umrigar… - Journal of the American …, 2022 - ACS Publications
The complex electronic structure and unusual potential energy curve of the chromium dimer
have fascinated scientists for decades, with agreement between theory and experiment so …

New density matrix renormalization group approaches for strongly correlated systems coupled with large environments

Y Xu, Y Cheng, Y Song, H Ma - Journal of Chemical Theory and …, 2023 - ACS Publications
Thanks to the high compression of the matrix product state (MPS) form of the wave function
and the efficient site-by-site iterative swee** optimization algorithm, the density matrix …

Reliably assessing the electronic structure of cytochrome P450 on today's classical computers and tomorrow's quantum computers

JJ Goings, A White, J Lee… - Proceedings of the …, 2022 - National Acad Sciences
An accurate assessment of how quantum computers can be used for chemical simulation,
especially their potential computational advantages, provides important context on how to …

Block2: A comprehensive open source framework to develop and apply state-of-the-art DMRG algorithms in electronic structure and beyond

H Zhai, HR Larsson, S Lee, ZH Cui, T Zhu… - The Journal of …, 2023 - pubs.aip.org
block2 is an open source framework to implement and perform density matrix
renormalization group and matrix product state algorithms. Out-of-the-box it supports the …

A perspective on sustainable computational chemistry software development and integration

R Di Felice, ML Mayes, RM Richard… - Journal of chemical …, 2023 - ACS Publications
The power of quantum chemistry to predict the ground and excited state properties of
complex chemical systems has driven the development of computational quantum chemistry …

Initial state preparation for quantum chemistry on quantum computers

S Fomichev, K Hejazi, MS Zini, M Kiser, J Fraxanet… - PRX Quantum, 2024 - APS
Quantum algorithms for ground-state energy estimation of chemical systems require a high-
quality initial state. However, initial state preparation is commonly either neglected entirely …

Is there evidence for exponential quantum advantage in quantum chemistry?

S Lee, J Lee, H Zhai, Y Tong, AM Dalzell… - arxiv preprint arxiv …, 2022 - arxiv.org
The idea to use quantum mechanical devices to simulate other quantum systems is
commonly ascribed to Feynman. Since the original suggestion, concrete proposals have …

Variational lang–firsov approach plus møller–plesset perturbation theory with applications to ab initio polariton chemistry

ZH Cui, A Mandal, DR Reichman - Journal of Chemical Theory …, 2024 - ACS Publications
We apply the Lang–Firsov (LF) transformation to electron–boson coupled Hamiltonians and
variationally optimize the transformation parameters and molecular orbital coefficients to …

Simulating models of challenging correlated molecules and materials on the Sycamore quantum processor

RN Tazhigulov, SN Sun, R Haghshenas, H Zhai… - PRX Quantum, 2022 - APS
Simulating complex molecules and materials is an anticipated application of quantum
devices. With the emergence of hardware designed to target strong quantum advantage in …