Recent progress in surface hop**: 2011–2015

L Wang, A Akimov, OV Prezhdo - The journal of physical chemistry …, 2016‏ - ACS Publications
Developed 25 years ago, Tully's fewest switches surface hop** (FSSH) has proven to be
the most popular approach for simulating quantum-classical dynamics in a broad variety of …

Quantum mechanical studies of large metal, metal oxide, and metal chalcogenide nanoparticles and clusters

A Fernando, KLDM Weerawardene… - Chemical …, 2015‏ - ACS Publications
Metal, metal oxide, and metal chalcogenide materials have a wide variety of applications.
For example, many metal clusters and nanoparticles are used as catalysts for reactions …

Structural disorder in higher-temperature phases increases charge carrier lifetimes in metal halide perovskites

R Shi, Q Fang, AS Vasenko, R Long… - Journal of the …, 2022‏ - ACS Publications
Solar cells and optoelectronic devices are exposed to heat that degrades performance.
Therefore, elucidating temperature-dependent charge carrier dynamics is essential for …

Low-frequency lattice phonons in halide perovskites explain high defect tolerance toward electron-hole recombination

W Chu, Q Zheng, OV Prezhdo, J Zhao, WA Saidi - Science advances, 2020‏ - science.org
Low-cost solution-based synthesis of metal halide perovskites (MHPs) invariably introduces
defects in the system, which could form Shockley-Read-Hall (SRH) electron-hole …

Two-dimensional trilayer heterostructures with cascade dual Z-schemes to achieve efficient hydrogen evolution reaction

XQ Wan, CL Yang, XH Li, YL Liu… - Journal of Materials …, 2024‏ - pubs.rsc.org
Cascade dual Z-schemes for photocatalytic overall water splitting for hydrogen production
are constructed for trilayer Bi/HfSeTe/ZrSe2, Bi/HfSeTe/ZrSe2, and InAs3/HfSeTe/ZrSe2 …

Rapid interlayer charge separation and extended carrier lifetimes due to spontaneous symmetry breaking in organic and mixed organic–inorganic Dion–Jacobson …

R Shi, R Long, WH Fang… - Journal of the American …, 2023‏ - ACS Publications
Promising alternatives to three-dimensional perovskites, two-dimensional (2D) layered
metal halide perovskites have proven their potential in optoelectronic applications due to …

Unravelling the Effects of Grain Boundary and Chemical Do** on Electron–Hole Recombination in CH3NH3PbI3 Perovskite by Time-Domain Atomistic Simulation

R Long, J Liu, OV Prezhdo - Journal of the American Chemical …, 2016‏ - ACS Publications
Advancing organohalide perovskite solar cells requires understanding of carrier dynamics.
Electron–hole recombination is a particularly important process because it constitutes a …

Advanced capabilities of the PYXAID program: integration schemes, decoherence effects, multiexcitonic states, and field-matter interaction

AV Akimov, OV Prezhdo - Journal of chemical theory and …, 2014‏ - ACS Publications
In our previous work [J. Chem. Theory Comput. 2013, 9, 4959], we introduced the PYXAID
program, developed for the purpose of performing nonadiabatic molecular dynamics …

Nuclear quantum effects prolong charge carrier lifetimes in hybrid organic–inorganic perovskites

Y Liu, R Long, WH Fang… - Journal of the American …, 2023‏ - ACS Publications
Hybrid organic–inorganic perovskites (HOIPs) contain light hydrogen atoms that exhibit
significant nuclear quantum effects (NQEs). We demonstrate that NQEs have a strong effect …

Ab initio nonadiabatic molecular dynamics of charge carriers in metal halide perovskites

W Li, Y She, AS Vasenko, OV Prezhdo - Nanoscale, 2021‏ - pubs.rsc.org
Photoinduced nonequilibrium processes in nanoscale materials play key roles in
photovoltaic and photocatalytic applications. This review summarizes recent theoretical …