Time‐resolved in situ monitoring of mechanochemical reactions

AAL Michalchuk, F Emmerling - … Chemie International Edition, 2022‏ - Wiley Online Library
Mechanochemical transformations offer environmentally benign synthesis routes, whilst
enhancing both the speed and selectivity of reactions. In this regard, mechanochemistry …

Toward Mechanistic Understanding of Mechanochemical Reactions Using Real-Time In Situ Monitoring

S Lukin, LS Germann, T Friščić… - Accounts of chemical …, 2022‏ - ACS Publications
Conspectus The past two decades have witnessed a rapid emergence of interest in
mechanochemistry–chemical and materials reactivity achieved or sustained by the action of …

Raman spectroscopy for real-time and in situ monitoring of mechanochemical milling reactions

S Lukin, K Užarević, I Halasz - Nature Protocols, 2021‏ - nature.com
Solid-state milling has emerged as an alternative, sustainable approach for preparing
virtually all classes of compounds and materials. In situ reaction monitoring is essential to …

Challenging the Ostwald rule of stages in mechanochemical cocrystallisation

LS Germann, M Arhangelskis, M Etter… - Chemical …, 2020‏ - pubs.rsc.org
Mechanochemistry provides an efficient, but still poorly understood route to synthesize and
screen for polymorphs of organic solids. We present a hitherto unexplored effect of the …

Mechanochemical Preparation of Active Pharmaceutical Ingredients Monitored by In Situ Raman Spectroscopy

I Sović, S Lukin, E Meštrović, I Halasz… - ACS …, 2020‏ - ACS Publications
The mechanochemical preparation of silver sulfadiazine and dantrolene, two marketed
active pharmaceutical ingredients, was investigated by in situ Raman spectroscopy. For the …

A review of recent developments for the in situ/operando characterization of nanoporous materials

H Petersen, C Weidenthaler - Inorganic Chemistry Frontiers, 2022‏ - pubs.rsc.org
This is a review on up-to-date in situ/operando methods for a comprehensive
characterization of nanoporous materials. The group of nanoporous materials is constantly …

Mechanochemical reaction kinetics scales linearly with impact energy

L Vugrin, M Carta, S Lukin, E Meštrović, F Delogu… - Faraday …, 2023‏ - pubs.rsc.org
Inelastic collisions of the milling media in ball milling provide energy to the reaction mixture
required for chemical transformations. However, movement of the milling media also results …

Enantiotropic inconstancy, crystalline solid solutions and co-crystal in the salicylic acid–anthranilic acid system

FL Nordstrom, SS Mohajerani, B Linehan… - Physical Chemistry …, 2022‏ - pubs.rsc.org
The phase boundaries and thermodynamic properties of crystal phases in the salicylic acid
(SA)–anthranilic acid (AA) system have been determined experimentally. The complete …

Isotope labeling reveals fast atomic and molecular exchange in mechanochemical milling reactions

S Lukin, M Tireli, T Stolar, D Barišić… - Journal of the …, 2019‏ - ACS Publications
Using tandem in situ monitoring and isotope-labeled solids, we reveal that
mechanochemical ball-milling overcomes inherently slow solid-state diffusion through …

Screening nature of the van der Waals density functional method: A review and analysis of the many-body physics foundation

P Hyldgaard, Y Jiao, V Shukla - Journal of Physics: Condensed …, 2020‏ - iopscience.iop.org
We review the screening nature and many-body physics foundation of the van der Waals
density functional (vdW-DF) method [Berland K et al 2015 Rep. Prog. Phys. 78 066501], a …