Multidimensional coherent spectroscopy of semiconductors

CL Smallwood, ST Cundiff - Laser & Photonics Reviews, 2018 - Wiley Online Library
Optical multidimensional coherent spectroscopy (MDCS) is a nonlinear spectroscopy
technique where a material is excited by a series of laser pulses to produce a spectrum as a …

Observing Multiexciton Correlations in Colloidal Semiconductor Quantum Dots via Multiple-Quantum Two-Dimensional Fluorescence Spectroscopy

S Mueller, J Lüttig, L Brenneis, D Oron, T Brixner - ACS nano, 2021 - ACS Publications
Correlations between excitons, that is, electron–hole pairs, have a great impact on the
optoelectronic properties of semiconductor quantum dots and thus are relevant for …

Controlled Coherent Coupling in a Quantum Dot Molecule Revealed by Ultrafast Four-Wave Mixing Spectroscopy

D Wigger, J Schall, M Deconinck, N Bart… - ACS …, 2023 - ACS Publications
Semiconductor quantum dot molecules are considered promising candidates for quantum
technological applications due to their wide tunability of optical properties and coverage of …

Controlled coherent-coupling and dynamics of exciton complexes in a MoSe2 monolayer

A Rodek, T Hahn, J Howarth, T Taniguchi… - 2D …, 2023 - iopscience.iop.org
Quantifying and controlling the coherent dynamics and couplings of optically active
excitations in solids is of paramount importance in fundamental research in condensed …

Inducing coherent quantum dot interactions

EW Martin, ST Cundiff - Physical Review B, 2018 - APS
We measure many-body interactions in isolated quantum dot states using double-quantum
multidimensional coherent spectroscopy. Few states are probed in a diffraction limited spot …

Roadmap on bio-nano-photonics

E Herkert, N Slesiona, ME Recchia, T Deckert… - Journal of …, 2021 - iopscience.iop.org
In the quest to decipher the chain of life from molecules to cells, the biological and
biophysical questions being asked increasingly demand techniques that are capable of …

[Књига][B] Optical multidimensional coherent spectroscopy

H Li, B Lomsadze, G Moody, C Smallwood, S Cundiff - 2023 - books.google.com
This book provides an introduction to optical multidimensional coherent spectroscopy, a
relatively new method of studying materials based on using ultrashort light pulses to perform …

Fluorescence-detected two-quantum photon echoes via cogwheel phase cycling

A Jayachandran, S Mueller… - The Journal of Physical …, 2022 - ACS Publications
Two-dimensional (2D) electronic spectroscopy can separate homogeneous and
inhomogeneous broadening. While established methods usually probe a photon-echo …

Destructive Photon Echo Formation in Six‐Wave Mixing Signals of a MoSe2 Monolayer

T Hahn, D Vaclavkova, M Bartos… - Advanced …, 2022 - Wiley Online Library
Monolayers of transition metal dichalcogenides display a strong excitonic optical response.
Additionally encapsulating the monolayer with hexagonal boron nitride allows to reach the …

OPA-driven hollow-core fiber as a tunable, broadband source for coherent multidimensional spectroscopy

C Sonnichsen, P Brosseau, C Reid… - Optics Express, 2021 - opg.optica.org
Despite the impressive abilities of coherent multi-dimensional spectroscopy (CMDS), its'
implementation is limited due to the complexity of continuum generation and required phase …