Thermal energy transport in oxide nuclear fuel

DH Hurley, A El-Azab, MS Bryan, MWD Cooper… - Chemical …, 2021 - ACS Publications
To efficiently capture the energy of the nuclear bond, advanced nuclear reactor concepts
seek solid fuels that must withstand unprecedented temperature and radiation extremes. In …

An integrated experimental and computational investigation of defect and microstructural effects on thermal transport in thorium dioxide

CA Dennett, WR Deskins, M Khafizov, Z Hua… - Acta Materialia, 2021 - Elsevier
Advanced nuclear reactor concepts aim to use fuels that must withstand unprecedented
temperature and radiation extremes. In these fuels, thermal energy transport under …

Dislocation loop evolution in Kr‐irradiated ThO2

L He, T Yao, K Bawane, M **, C Jiang… - Journal of the …, 2022 - Wiley Online Library
The early stage of microstructural evolution of ThO2, under krypton irradiation at 600, 800,
and 1000° C, was investigated using in situ transmission electron microscopy (TEM) …

Phonon Thermal Transport in via Self-Consistent Perturbation Theory

S Zhou, E **ao, H Ma, K Gofryk, C Jiang, ME Manley… - Physical Review Letters, 2024 - APS
Computing thermal transport from first-principles in UO 2 is complicated due to the
challenges associated with Mott physics. Here, we use irreducible derivative approaches to …

Capturing the ground state of uranium dioxide from first principles: Crystal distortion, magnetic structure, and phonons

S Zhou, H Ma, E **ao, K Gofryk, C Jiang, ME Manley… - Physical Review B, 2022 - APS
Uranium dioxide (UO 2) remains a formidable challenge for first-principles approaches due
to the complex interplay among spin-orbit coupling, Mott physics, magnetic ordering, and …

Generalized quasiharmonic approximation via space group irreducible derivatives

MA Mathis, A Khanolkar, L Fu, MS Bryan, CA Dennett… - Physical Review B, 2022 - APS
The quasiharmonic approximation (QHA) is the simplest nontrivial approximation for
interacting phonons under constant pressure, bringing the effects of anharmonicity into …

TEM characterization of dislocation loops in proton irradiated single crystal ThO2

K Bawane, X Liu, T Yao, M Khafizov, A French… - Journal of Nuclear …, 2021 - Elsevier
This work focuses on the full characterization of dislocation loops induced by proton
irradiation in single-crystal ThO 2. Irradiation was performed using 2 MeV H+ ions with …

Structural dynamics of Schottky and Frenkel defects in ThO 2: a density-functional theory study

S Moxon, J Skelton, ST Joshua, J Flitcroft… - Journal of Materials …, 2022 - pubs.rsc.org
Thorium dioxide (ThO2) is a promising alternative to mixed-oxide nuclear fuels due to its
longer fuel cycle and resistance to proliferation. Understanding the thermal properties, in …

First principles investigations for structural, electronic, optical and elastic properties of Ag2BeSn (S/Se) 4 chalcogenide in kesterite and stannite phases with theoretical …

A Srivastava, A Mannodi-Kanakkithodi… - Physica B: Condensed …, 2023 - Elsevier
In the present work, density functional theory based computational analysis is carried out for
structural, electronic, optical, and mechanical properties of novel chalcogenide Ag 2 BeSn …

Inferring relative dose-dependent color center populations in proton irradiated thoria single crystals using optical spectroscopy

A Khanolkar, CA Dennett, Z Hua, JM Mann… - Physical Chemistry …, 2022 - pubs.rsc.org
We have utilized photoluminescence spectroscopy and optical ellipsometry to characterize
the dose-dependence of the photoluminescence emission intensity and changes in optical …