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Methane activation by heterogeneous catalysis
R Horn, R Schlögl - Catalysis Letters, 2015 - Springer
Methane activation by heterogeneous catalysis will play a key role to secure the supply of
energy, chemicals and fuels in the future. Methane is the main constituent of natural gas and …
energy, chemicals and fuels in the future. Methane is the main constituent of natural gas and …
Chemistry with methane: concepts rather than recipes
Four seemingly simple transformations related to the chemistry of methane will be
addressed from mechanistic and conceptual points of view: 1) metal‐mediated …
addressed from mechanistic and conceptual points of view: 1) metal‐mediated …
Thermal hydrogen‐atom transfer from methane: the role of radicals and spin states in oxo‐cluster chemistry
Abstract Hydrogen‐atom transfer (HAT), as one of the fundamental reactions in chemistry, is
investigated with state‐of‐the‐art gas‐phase experiments in conjunction with computational …
investigated with state‐of‐the‐art gas‐phase experiments in conjunction with computational …
Electronic effects on room-temperature, gas-phase C–H Bond activations by cluster oxides and metal carbides: The methane challenge
This Perspective discusses a story of one molecule (methane), a few metal-oxide cationic
clusters (MOCCs), dopants, metal-carbide cations, oriented-electric fields (OEFs), and a …
clusters (MOCCs), dopants, metal-carbide cations, oriented-electric fields (OEFs), and a …
C–H bond activation by oxygen-centered radicals over atomic clusters
Saturated hydrocarbons, or alkanes, are major constituents of natural gas and oil. Directly
transforming alkanes into more complex organic compounds is a value-adding process, but …
transforming alkanes into more complex organic compounds is a value-adding process, but …
Do** effects in cluster‐mediated bond activation
Gas‐phase investigations of judiciously doped oxide clusters permit to address fundamental
challenges related to, for example, the low‐temperature oxidation of CO or the selective …
challenges related to, for example, the low‐temperature oxidation of CO or the selective …
Thermal Methane Conversion to Formaldehyde Promoted by Single Platinum Atoms in PtAl2O4− Cluster Anions
YX Zhao, ZY Li, Z Yuan, XN Li… - Angewandte Chemie …, 2014 - Wiley Online Library
Identification and mechanistic study of thermal methane conversion mediated by gas‐phase
species is important for finding potentially useful routes for direct methane transformation …
species is important for finding potentially useful routes for direct methane transformation …
Characterization and reactivity of oxygen-centred radicals over transition metal oxide clusters
We introduce chemical structures and reactivity of oxygen-centred radicals (O−˙) over
transition metal oxide (TMO) clusters based on mass spectrometric and density functional …
transition metal oxide (TMO) clusters based on mass spectrometric and density functional …
Effects of ligands, cluster size, and charge state in gas-phase catalysis: a happy marriage of experimental and computational studies
We present selected examples of gas-phase reactions which are of timely interest for the
activation of small molecules. Due to the very nature of the experiments, detailed insight in …
activation of small molecules. Due to the very nature of the experiments, detailed insight in …
Thermal hydrogen-atom transfer from methane: A mechanistic exercise
Hydrogen-atom transfer (HAT) constitutes a key process in a broad range of chemical
transformations as it covers heterogeneous, homogeneous, and enzymatic reactions. While …
transformations as it covers heterogeneous, homogeneous, and enzymatic reactions. While …