Carbon nitride based materials: more than just a support for single-atom catalysis

GFSR Rocha, MAR da Silva, A Rogolino… - Chemical Society …, 2023 - pubs.rsc.org
Recently, the missing link between homogeneous and heterogeneous catalysis has been
found and it was named single-atom catalysis (SAC). However, the SAC field still faces …

Polymer photocatalysts for solar-to-chemical energy conversion

T Banerjee, F Podjaski, J Kröger, BP Biswal… - Nature Reviews …, 2021 - nature.com
Solar-to-chemical energy conversion for the generation of high-energy chemicals is one of
the most viable solutions to the quest for sustainable energy resources. Although long …

Understanding the unique S-scheme charge migration in triazine/heptazine crystalline carbon nitride homojunction

F Li, X Yue, Y Liao, L Qiao, K Lv, Q **ang - Nature Communications, 2023 - nature.com
Understanding charge transfer dynamics and carrier separation pathway is challenging due
to the lack of appropriate characterization strategies. In this work, a crystalline …

S-scheme heterojunction of crystalline carbon nitride nanosheets and ultrafine WO3 nanoparticles for photocatalytic CO2 reduction

G Chen, Z Zhou, B Li, X Lin, C Yang, Y Fang… - Journal of …, 2024 - Elsevier
Highly crystalline carbon nitride polymers have shown great opportunities in overall water
photosplitting; however, their mission in light-driven CO 2 conversion remains to be …

Bottom‐up synthesis of single‐crystalline poly (triazine imide) nanosheets for photocatalytic overall water splitting

Q Wang, G Zhang, W **ng, Z Pan, D Zheng… - Angewandte …, 2023 - Wiley Online Library
Abstract Poly (triazine imide)(PTI/Li+ Cl−), one of the crystalline versions of polymeric carbon
nitrides, holds great promise for photocatalytic overall water splitting. In principle, the …

Improved charge separation in poly (heptazine‐triazine) imides with semi‐coherent interfaces for photocatalytic hydrogen evolution

J Zhang, X Liang, C Zhang, L Lin… - Angewandte Chemie …, 2022 - Wiley Online Library
The construction of heterojunctions is a promising manner to accelerate the separation and
transfer of the charge carriers at the interface. Herein, a binary poly (heptazine‐triazine) …

Homogeneous Carbon/Potassium‐Incorporation Strategy for Synthesizing Red Polymeric Carbon Nitride Capable of Near‐Infrared Photocatalytic H2 Production

Y Xu, M Fan, W Yang, Y **ao, L Zeng, X Wu… - Advanced …, 2021 - Wiley Online Library
The efficient utilization of near‐infrared (NIR) light for photocatalytic hydrogen generation is
vitally important to both solar hydrogen energy and hydrogen medicine, but remains a …

Molecular-level insights on the reactive facet of carbon nitride single crystals photocatalysing overall water splitting

L Lin, Z Lin, J Zhang, X Cai, W Lin, Z Yu, X Wang - Nature Catalysis, 2020 - nature.com
Unraveling how reactive facets promote photocatalysis at the molecular level remains a
grand challenge, while identification of the reactive facets can provide guidelines for …

Atomically dispersed low-valent Au boosts photocatalytic hydroxyl radical production

Z Teng, H Yang, Q Zhang, W Cai, YR Lu, K Kato… - Nature Chemistry, 2024 - nature.com
Providing affordable, safe drinking water and universal sanitation poses a grand societal
challenge. Here we developed atomically dispersed Au on potassium-incorporated …

Fully condensed poly (triazine imide) crystals: extended π‐conjugation and structural defects for overall water splitting

M Liu, C Wei, H Zhuzhang, J Zhou… - Angewandte Chemie …, 2022 - Wiley Online Library
Conventional polymerization for the synthesis of carbon nitride usually generates
amorphous heptazine‐based melon with an abundance of undesired structural defects …