First demonstrated in 1994, femtosecond stimulated Raman scattering (FSRS) has gained
popularity since the early 2000s as an ultrafast pump–probe vibrational spectroscopy …

Femtosecond stimulated Raman spectroscopy (FSRS) is an ultrafast nonlinear optical
technique that provides vibrational structural information with high temporal (sub‐50 fs) …

Crossings of electronic potential energy surfaces in nuclear configuration space, known as
conical intersections, determine the rates and outcomes of a large class of photochemical …

Computational spectroscopy is becoming a mandatory tool for the interpretation of the
complex, and often congested, spectral maps delivered by modern non-linear multi-pulse …

Chemistry studies the composition, structure, properties, and transformation of matter. A
mechanistic understanding of the pertinent processes is required to translate fundamental …

The structure–function relationships of biomolecules have captured the interest and
imagination of the scientific community and general public since the field of structural …

Ultrafast reactions activated by light absorption are governed by multidimensional excited-
state (ES) potential energy surfaces (PESs), which describe how the molecular potential …

The quest for capturing molecular movies of functional systems has motivated scientists and
engineers for decades. A fundamental understanding of electronic and nuclear motions, two …

Photophysical and photochemical processes are ruled by the interplay between transient
vibrational and electronic degrees of freedom, which are ultimately determined by the …

Excited state vibrations are crucial for determining the photophysical and photochemical
properties of molecular compounds. Stimulated Raman scattering can coherently stimulate …