Iron and manganese oxo complexes, oxo wall and beyond

VA Larson, B Battistella, K Ray, N Lehnert… - Nature Reviews …, 2020 - nature.com
High-valent metal–oxo species with multiply-bonded M–O groups have been proposed as
key intermediates in many biological and abiological catalytic oxidation reactions. These …

Bioinspired Nonheme Iron Catalysts for C–H and C C Bond Oxidation: Insights into the Nature of the Metal-Based Oxidants

WN Oloo, L Que Jr - Accounts of chemical research, 2015 - ACS Publications
Conspectus Recent efforts to design synthetic iron catalysts for the selective and efficient
oxidation of C–H and C C bonds have been inspired by a versatile family of nonheme iron …

Trap** a Highly Reactive Nonheme Iron Intermediate That Oxygenates Strong C H Bonds with Stereoretention

J Serrano-Plana, WN Oloo… - Journal of the …, 2015 - ACS Publications
An unprecedentedly reactive iron species (2) has been generated by reaction of excess
peracetic acid with a mononuclear iron complex [FeII (CF3SO3) 2 (PyNMe3)](1) at cryogenic …

Artificial nonheme iron and manganese oxygenases for enantioselective olefin epoxidation and alkane hydroxylation reactions

J Chen, Z Jiang, S Fukuzumi, W Nam… - Coordination Chemistry …, 2020 - Elsevier
The development of sustainable enantioselective olefin epoxidation and alkane oxidation
reactions under environmentally friendly conditions is an ultimate goal that has long been …

Oxidation of alkane and alkene moieties with biologically inspired nonheme iron catalysts and hydrogen peroxide: from free radicals to stereoselective transformations

G Olivo, O Cussó, M Borrell, M Costas - JBIC Journal of Biological …, 2017 - Springer
The selective oxidation of hydrocarbons is a challenging reaction for synthetic chemists, but
common in nature. Iron oxygenases activate the O–O bond of dioxygen to perform oxidation …

Biologically inspired non-heme iron-catalysts for asymmetric epoxidation; design principles and perspectives

O Cussó, X Ribas, M Costas - Chemical Communications, 2015 - pubs.rsc.org
Iron coordination complexes with nitrogen and oxygen donor ligands have long since been
known to react with peroxides producing powerful oxidizing species. These compounds can …

Biomimetic metal-oxidant adducts as active oxidants in oxidation reactions

M Guo, YM Lee, S Fukuzumi, W Nam - Coordination Chemistry Reviews, 2021 - Elsevier
Catalytic oxidation reactions are pivotal transformations in living creatures and chemical
industries, in which metal-oxygen intermediates, including high-valent metal-oxo species …

Charged droplet-driven fast formation of nickel–iron (oxy) hydroxides with rich oxygen defects for boosting overall water splitting

J Dong, Y Wang, Q Jiang, ZA Nan, FR Fan… - Journal of Materials …, 2021 - pubs.rsc.org
NiFe (oxy) hydroxides (NiFeOOH) are considered as one of the most efficient
electrocatalysts for water splitting. Although several strategies recently have been …

Spectroscopic and DFT Characterization of a Highly Reactive Nonheme FeV–Oxo Intermediate

R Fan, J Serrano-Plana, WN Oloo… - Journal of the …, 2018 - ACS Publications
The reaction of [(PyNMe3) FeII (CF3SO3) 2], 1, with excess peracetic acid at− 40° C
generates a highly reactive intermediate, 2b (PAA), that has the fastest rate to date for …

Speciation in iron epoxidation catalysis: A perspective on the discovery and role of non-heme iron (III)-hydroperoxo species in iron-catalyzed oxidation reactions

SM Hölzl, PJ Altmann, JW Kück, FE Kühn - Coordination Chemistry …, 2017 - Elsevier
Oxidation reactions catalyzed by enzymes with central iron atoms are essential to life. The
nature of these systems has evoked great interest to understand and model their reactivity …