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Engineering exciton dynamics with synthetic DNA scaffolds
Conspectus Excitons are the molecular-scale currency of electronic energy. Control over
excitons enables energy to be directed and harnessed for light harvesting, electronics, and …
excitons enables energy to be directed and harnessed for light harvesting, electronics, and …
Develo** FRET networks for sensing
Förster resonance energy transfer (FRET) is a widely used fluorescence-based sensing
mechanism. To date, most implementations of FRET sensors have relied on a discrete donor …
mechanism. To date, most implementations of FRET sensors have relied on a discrete donor …
Engineering couplings for exciton transport using synthetic DNA scaffolds
Control over excitons enables electronic energy to be harnessed and transported for light
harvesting and molecular electronics. Such control requires nanoscale precision over the …
harvesting and molecular electronics. Such control requires nanoscale precision over the …
Exciton delocalization in indolenine squaraine aggregates templated by DNA holliday junction scaffolds
OA Mass, CK Wilson, SK Roy, MS Barclay… - The Journal of …, 2020 - ACS Publications
Exciton delocalization plays a prominent role in the photophysics of molecular aggregates,
ultimately governing their particular function or application. Deoxyribonucleic acid (DNA) is a …
ultimately governing their particular function or application. Deoxyribonucleic acid (DNA) is a …
Optically accessible long-lived electronic biexcitons at room temperature in strongly coupled H-aggregates
Photon absorption is the first process in light harvesting. Upon absorption, the photon
redistributes electrons in the materials to create a Coulombically bound electron-hole pair …
redistributes electrons in the materials to create a Coulombically bound electron-hole pair …
Tuning optical absorption and emission using strongly coupled dimers in programmable DNA scaffolds
Molecular materials for light harvesting, computing, and fluorescence imaging require
nanoscale integration of electronically active subunits. Variation in the optical absorption …
nanoscale integration of electronically active subunits. Variation in the optical absorption …
Influence of hydrophobicity on excitonic coupling in DNA-templated indolenine squaraine dye aggregates
OA Mass, CK Wilson, G Barcenas… - The Journal of …, 2022 - ACS Publications
Control over the strength of excitonic coupling in molecular dye aggregates is a substantial
factor for the development of technologies such as light harvesting, optoelectronics, and …
factor for the development of technologies such as light harvesting, optoelectronics, and …
Tuning between quenching and energy transfer in DNA-templated heterodimer aggregates
Molecular excitons, which propagate spatially via electronic energy transfer, are central to
numerous applications including light harvesting, organic optoelectronics, and nanoscale …
numerous applications including light harvesting, organic optoelectronics, and nanoscale …
Two‐Dimensional Excitonic Networks Directed by DNA Templates as an Efficient Model Light‐Harvesting and Energy Transfer System
Photosynthetic organisms organize discrete light‐harvesting complexes into large‐scale
networks to facilitate efficient light collection and utilization. Inspired by nature, herein …
networks to facilitate efficient light collection and utilization. Inspired by nature, herein …
First-principles studies of substituent effects on squaraine dyes
G Barcenas, A Biaggne, OA Mass, CK Wilson… - RSC …, 2021 - pubs.rsc.org
Dye molecules that absorb light in the visible region are key components in many
applications, including organic photovoltaics, biological fluorescent labeling, super …
applications, including organic photovoltaics, biological fluorescent labeling, super …