Using X-ray free-electron lasers for spectroscopy of molecular catalysts and metalloenzymes

U Bergmann, J Kern, RW Schoenlein, P Wernet… - Nature Reviews …, 2021 - nature.com
The metal centres in metalloenzymes and molecular catalysts are responsible for the
rearrangement of atoms and electrons during complex chemical reactions, and they enable …

Recent advances in ultrafast X-ray sources

R Schoenlein, T Elsaesser… - … of the Royal …, 2019 - royalsocietypublishing.org
Over more than a century, X-rays have transformed our understanding of the fundamental
structure of matter and have been an indispensable tool for chemistry, physics, biology …

Attosecond coherent control of electronic wave packets in two-colour photoionization using a novel timing tool for seeded free-electron laser

PK Maroju, M Di Fraia, O Plekan, M Bonanomi… - Nature …, 2023 - nature.com
In ultrafast spectroscopy, the temporal resolution of time-resolved experiments depends on
the duration of the pump and probe pulses, and on the control and characterization of their …

The MING proposal at SHINE: Megahertz cavity enhanced X-ray generation

NS Huang, ZP Liu, BJ Deng, ZH Zhu, SH Li… - Nuclear Science and …, 2023 - Springer
The cavity-based X-ray free-electron laser (XFEL) has promise in producing fully coherent
pulses with a bandwidth of a few meV and very stable intensity, whereas the currently …

Attosecond pulse sha** using a seeded free-electron laser

PK Maroju, C Grazioli, M Di Fraia, M Moioli, D Ertel… - Nature, 2020 - nature.com
Attosecond pulses are central to the investigation of valence-and core-electron dynamics on
their natural timescales,–. The reproducible generation and characterization of attosecond …

Femtosecond polarization sha** of free-electron laser pulses

G Perosa, J Wätzel, D Garzella, E Allaria… - Physical Review Letters, 2023 - APS
We demonstrate the generation of extreme-ultraviolet (XUV) free-electron laser (FEL) pulses
with time-dependent polarization. To achieve polarization modulation on a femtosecond …

Tracking the ultraviolet-induced photochemistry of thiophenone during and after ultrafast ring opening

S Pathak, LM Ibele, R Boll, C Callegari… - Nature …, 2020 - nature.com
Photoinduced isomerization reactions lie at the heart of many chemical processes in nature.
The mechanisms of such reactions are determined by a delicate interplay of coupled …

Generation and measurement of intense few-femtosecond superradiant extreme-ultraviolet free-electron laser pulses

NS Mirian, M Di Fraia, S Spampinati, F Sottocorona… - Nature …, 2021 - nature.com
Free-electron lasers producing ultrashort pulses with high peak power promise to extend
ultrafast non-linear spectroscopic techniques into the extreme-ultraviolet–X-ray regime. Key …

Coherent and ultrashort soft x-ray pulses from echo-enabled harmonic cascade free-electron lasers

C Feng, T Liu, S Chen, K Zhou, K Zhang, Z Qi, D Gu… - Optica, 2022 - opg.optica.org
It is a long-standing challenge for laser technologies to generate intense fully coherent
pulses in the x-ray regime. Here, we demonstrate an external seeding mechanism, termed …

Generation of entanglement using a short-wavelength seeded free-electron laser

S Nandi, A Stenquist, A Papoulia, E Olofsson… - Science …, 2024 - science.org
Quantum entanglement between the degrees of freedom encountered in the classical world
is challenging to observe due to the surrounding environment. To elucidate this issue, we …