Using X-ray free-electron lasers for spectroscopy of molecular catalysts and metalloenzymes
The metal centres in metalloenzymes and molecular catalysts are responsible for the
rearrangement of atoms and electrons during complex chemical reactions, and they enable …
rearrangement of atoms and electrons during complex chemical reactions, and they enable …
Recent advances in ultrafast X-ray sources
Over more than a century, X-rays have transformed our understanding of the fundamental
structure of matter and have been an indispensable tool for chemistry, physics, biology …
structure of matter and have been an indispensable tool for chemistry, physics, biology …
Attosecond coherent control of electronic wave packets in two-colour photoionization using a novel timing tool for seeded free-electron laser
In ultrafast spectroscopy, the temporal resolution of time-resolved experiments depends on
the duration of the pump and probe pulses, and on the control and characterization of their …
the duration of the pump and probe pulses, and on the control and characterization of their …
The MING proposal at SHINE: Megahertz cavity enhanced X-ray generation
NS Huang, ZP Liu, BJ Deng, ZH Zhu, SH Li… - Nuclear Science and …, 2023 - Springer
The cavity-based X-ray free-electron laser (XFEL) has promise in producing fully coherent
pulses with a bandwidth of a few meV and very stable intensity, whereas the currently …
pulses with a bandwidth of a few meV and very stable intensity, whereas the currently …
Attosecond pulse sha** using a seeded free-electron laser
Attosecond pulses are central to the investigation of valence-and core-electron dynamics on
their natural timescales,–. The reproducible generation and characterization of attosecond …
their natural timescales,–. The reproducible generation and characterization of attosecond …
Femtosecond polarization sha** of free-electron laser pulses
We demonstrate the generation of extreme-ultraviolet (XUV) free-electron laser (FEL) pulses
with time-dependent polarization. To achieve polarization modulation on a femtosecond …
with time-dependent polarization. To achieve polarization modulation on a femtosecond …
Tracking the ultraviolet-induced photochemistry of thiophenone during and after ultrafast ring opening
Photoinduced isomerization reactions lie at the heart of many chemical processes in nature.
The mechanisms of such reactions are determined by a delicate interplay of coupled …
The mechanisms of such reactions are determined by a delicate interplay of coupled …
Generation and measurement of intense few-femtosecond superradiant extreme-ultraviolet free-electron laser pulses
NS Mirian, M Di Fraia, S Spampinati, F Sottocorona… - Nature …, 2021 - nature.com
Free-electron lasers producing ultrashort pulses with high peak power promise to extend
ultrafast non-linear spectroscopic techniques into the extreme-ultraviolet–X-ray regime. Key …
ultrafast non-linear spectroscopic techniques into the extreme-ultraviolet–X-ray regime. Key …
Coherent and ultrashort soft x-ray pulses from echo-enabled harmonic cascade free-electron lasers
C Feng, T Liu, S Chen, K Zhou, K Zhang, Z Qi, D Gu… - Optica, 2022 - opg.optica.org
It is a long-standing challenge for laser technologies to generate intense fully coherent
pulses in the x-ray regime. Here, we demonstrate an external seeding mechanism, termed …
pulses in the x-ray regime. Here, we demonstrate an external seeding mechanism, termed …
Generation of entanglement using a short-wavelength seeded free-electron laser
Quantum entanglement between the degrees of freedom encountered in the classical world
is challenging to observe due to the surrounding environment. To elucidate this issue, we …
is challenging to observe due to the surrounding environment. To elucidate this issue, we …