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Fresh look at electron-transfer mechanisms via the donor/acceptor bindings in the critical encounter complex
Seminal insights provided by the iconic RS Mulliken and his “charge-transfer” theory, H.
Taube and his “outer/inner-sphere” mechanisms, RA Marcus and his “two-state non …
Taube and his “outer/inner-sphere” mechanisms, RA Marcus and his “two-state non …
Kinetics of electron-transfer reactions at nanoelectrodes
The kinetics of several fast heterogeneous electron-transfer reactions were investigated by
steady-state voltammetry at nanoelectrodes and scanning electrochemical microscopy …
steady-state voltammetry at nanoelectrodes and scanning electrochemical microscopy …
Resonating valence-bond ground state in a phenalenyl-based neutral radical conductor
An organic material composed of neutral free radicals based on the spirobiphenalenyl
system exhibits a room temperature conductivity of 0.3 siemens per centimeter and a high …
system exhibits a room temperature conductivity of 0.3 siemens per centimeter and a high …
Intermolecular π-to-π bonding between stacked aromatic dyads. Experimental and theoretical binding energies and near-IR optical transitions for phenalenyl radical …
The high symmetry and stability of phenalenyl systems, both as the planar π-radical (P•) and
as the π-cation (P+), are desirable characteristics of prototypical aromatic donor/acceptor …
as the π-cation (P+), are desirable characteristics of prototypical aromatic donor/acceptor …
Stable (long-bonded) dimers via the quantitative self-association of different cationic, anionic, and uncharged π-radicals: Structures, energetics, and optical transitions
Unusual dimers with wide interplanar separations, that is, very long bonds with d D≈ 3.05 Å,
are common to the spontaneous self-association of various organic π-radicals in solution …
are common to the spontaneous self-association of various organic π-radicals in solution …
Electron delocalization in a rigid cofacial naphthalene‐1, 8: 4, 5‐bis (dicarboximide) dimer
Investigating through‐space electronic communication between discrete cofacially oriented
aromatic π‐systems is fundamental to understanding assemblies as diverse as double …
aromatic π‐systems is fundamental to understanding assemblies as diverse as double …
Donor− acceptor (electronic) coupling in the precursor complex to organic electron transfer: intermolecular and intramolecular self-exchange between phenothiazine …
Intermolecular electron transfer (ET) between the free phenothiazine donor (PH) and its
cation radical (PH•+) proceeds via the [1: 1] precursor complex (PH) 2•+ which is transiently …
cation radical (PH•+) proceeds via the [1: 1] precursor complex (PH) 2•+ which is transiently …
Molecular and electronic structures of the long-bonded π-dimers of tetrathiafulvalene cation-radical in intermolecular electron transfer and in (solid-state) conductivity
Tetrathiafulvalene (TTF) as the prototypical electron donor for solid-state (electronics)
applications is converted to the unusual cation-radical salt, TTF+• CB-(where CB-is the non …
applications is converted to the unusual cation-radical salt, TTF+• CB-(where CB-is the non …
Scanning electrochemical microscopy with gold nanotips: the effect of electrode material on electron transfer rates
The disk-type, polished Au nanoelectrodes were prepared, characterized, and used as tips
in the scanning electrochemical microscope (SECM). Kinetic parameters were measured for …
in the scanning electrochemical microscope (SECM). Kinetic parameters were measured for …
Electron hop** in π-stacked covalent and self-assembled perylene diimides observed by ENDOR spectroscopy
MJ Tauber, RF Kelley, JM Giaimo… - Journal of the …, 2006 - ACS Publications
We have carried out room-temperature, solution-phase electron paramagnetic resonance
and electron− nuclear double resonance studies on a series of radical anions based upon …
and electron− nuclear double resonance studies on a series of radical anions based upon …