Exploiting chemistry and molecular systems for quantum information science

MR Wasielewski, MDE Forbes, NL Frank… - Nature Reviews …, 2020 - nature.com
The power of chemistry to prepare new molecules and materials has driven the quest for
new approaches to solve problems having global societal impact, such as in renewable …

Recent advances and perspectives on nonadiabatic mixed quantum–classical dynamics

R Crespo-Otero, M Barbatti - Chemical reviews, 2018 - ACS Publications
Nonadiabatic mixed quantum–classical (NA-MQC) dynamics methods form a class of
computational theoretical approaches in quantum chemistry tailored to investigate the time …

Non-adiabatic excited-state molecular dynamics: Theory and applications for modeling photophysics in extended molecular materials

TR Nelson, AJ White, JA Bjorgaard, AE Sifain… - Chemical …, 2020 - ACS Publications
Optically active molecular materials, such as organic conjugated polymers and biological
systems, are characterized by strong coupling between electronic and vibrational degrees of …

Charge transport in molecular materials: An assessment of computational methods

H Oberhofer, K Reuter, J Blumberger - Chemical reviews, 2017 - ACS Publications
The booming field of molecular electronics has fostered a surge of computational research
on electronic properties of organic molecular solids. In particular, with respect to a …

Newton‐X: a surface‐hop** program for nonadiabatic molecular dynamics

M Barbatti, M Ruckenbauer, F Plasser… - Wiley …, 2014 - Wiley Online Library
The N ewton‐X program is a general‐purpose program package for excited‐state molecular
dynamics, including nonadiabatic methods. Its modular design allows N ewton‐X to be …

Decoherence-induced surface hop**

HM Jaeger, S Fischer, OV Prezhdo - The Journal of chemical physics, 2012 - pubs.aip.org
A simple surface hop** method for nonadiabatic molecular dynamics is developed. The
method derives from a stochastic modeling of the time-dependent Schrödinger and master …

Unravelling the Effects of Grain Boundary and Chemical Do** on Electron–Hole Recombination in CH3NH3PbI3 Perovskite by Time-Domain Atomistic Simulation

R Long, J Liu, OV Prezhdo - Journal of the American Chemical …, 2016 - ACS Publications
Advancing organohalide perovskite solar cells requires understanding of carrier dynamics.
Electron–hole recombination is a particularly important process because it constitutes a …

Understanding the surface hop** view of electronic transitions and decoherence

JE Subotnik, A Jain, B Landry, A Petit… - Annual review of …, 2016 - annualreviews.org
We present a current, up-to-date review of the surface hop** methodology for solving
nonadiabatic problems, 25 years after Tully published the fewest switches surface hop** …

Mixed quantum–classical dynamics

JC Tully - Faraday Discussions, 1998 - pubs.rsc.org
We present a unified derivation of the mean-field (Ehrenfest) and surface-hop**
approaches to mixed quantum–classical dynamics that elucidates the underlying …

Equation-of-Motion Methods for the Calculation of Femtosecond Time-Resolved 4-Wave-Mixing and N-Wave-Mixing Signals

MF Gelin, L Chen, W Domcke - Chemical Reviews, 2022 - ACS Publications
Femtosecond nonlinear spectroscopy is the main tool for the time-resolved detection of
photophysical and photochemical processes. Since most systems of chemical interest are …