Metal–organic frameworks in heterogeneous catalysis: recent progress, new trends, and future perspectives

A Bavykina, N Kolobov, IS Khan, JA Bau… - Chemical …, 2020 - ACS Publications
More than 95%(in volume) of all of today's chemical products are manufactured through
catalytic processes, making research into more efficient catalytic materials a thrilling and …

Power of infrared and raman spectroscopies to characterize metal-organic frameworks and investigate their interaction with guest molecules

KI Hadjiivanov, DA Panayotov, MY Mihaylov… - Chemical …, 2020 - ACS Publications
The variety of functionalities and porous structures inherent to metal-organic frameworks
(MOFs) together with the facile tunability of their properties makes these materials suitable …

Surface coordination chemistry of atomically dispersed metal catalysts

R Qin, K Liu, Q Wu, N Zheng - Chemical Reviews, 2020 - ACS Publications
Atomically dispersed metal catalysts (ADCs), as an emerging class of heterogeneous
catalysts, have been widely investigated during the past two decades. The atomic dispersion …

Catalysis by metal organic frameworks: perspective and suggestions for future research

D Yang, BC Gates - Acs Catalysis, 2019 - ACS Publications
Metal organic frameworks (MOFs) have drawn wide attention as potential catalysts, offering
high densities of catalytic sites in high-area porous solids, some with stabilities at high …

Defect engineering: tuning the porosity and composition of the metal–organic framework UiO-66 via modulated synthesis

GC Shearer, S Chavan, S Bordiga, S Svelle… - Chemistry of …, 2016 - ACS Publications
Presented in this paper is a deep investigation into the defect chemistry of UiO-66 when
synthesized in the presence of monocarboxylic acid modulators under the most commonly …

Modulating coordination environment of single-atom catalysts and their proximity to photosensitive units for boosting MOF photocatalysis

X Ma, H Liu, W Yang, G Mao, L Zheng… - Journal of the American …, 2021 - ACS Publications
Well-organized photosensitive units and catalytic sites in proximity are crucial for improving
charge separation efficiency and boosting photocatalysis. Herein, a general and facile …

Secondary building units as the turning point in the development of the reticular chemistry of MOFs

MJ Kalmutzki, N Hanikel, OM Yaghi - Science advances, 2018 - science.org
The secondary building unit (SBU) approach was a turning point in the discovery of
permanently porous metal-organic frameworks (MOFs) and in launching the field of reticular …

Machine learning the quantum-chemical properties of metal–organic frameworks for accelerated materials discovery

AS Rosen, SM Iyer, D Ray, Z Yao, A Aspuru-Guzik… - Matter, 2021 - cell.com
The modular nature of metal–organic frameworks (MOFs) enables synthetic control over
their physical and chemical properties, but it can be difficult to know which MOFs would be …

Metal–organic frameworks for the removal of toxic industrial chemicals and chemical warfare agents

NS Bobbitt, ML Mendonca, AJ Howarth… - Chemical Society …, 2017 - pubs.rsc.org
Owing to the vast diversity of linkers, nodes, and topologies, metal–organic frameworks can
be tailored for specific tasks, such as chemical separations or catalysis. Accordingly, these …

Destruction of chemical warfare agents using metal–organic frameworks

JE Mondloch, MJ Katz, WC Isley Iii, P Ghosh, P Liao… - Nature materials, 2015 - nature.com
Chemical warfare agents containing phosphonate ester bonds are among the most toxic
chemicals known to mankind. Recent global military events, such as the conflict and …