An asymmetric substrate-controlled Morita–Baylis–Hillman reaction as approach for the synthesis of pyrrolizidinones and pyrrolizidines

KR Luna-Freire, JPS Scaramal, JALC Resende… - Tetrahedron, 2014 - Elsevier
We describe herein an approach to the total synthesis of functionalized pyrrolizidinones and
pyrrolizidines. The synthetic sequence is based on a highly stereoselective substrate …

[HTML][HTML] (1S, 2E, 6R, 7aR)-1, 6-Dihydroxy-2-(4-nitrobenzylidene)-2, 3, 5, 6, 7, 7a-hexahydro-1H-pyrrolizin-3-one

FL Oliveira, KRL Freire, R Aparicio, F Coelho - Structure Reports, 2012 - journals.iucr.org
The crystal structure of the title compound, C14H14N2O5, contains two distinct conformers
in the asymmetric unit. The compound has three defined stereocenters, two of them …

(1S, 2E, 6R, 7aR)-2-Benzylidene-1, 6-dihydroxy-2, 3, 5, 6, 7, 7a-hexahydro-1H-pyrrolizin-3-one

FL Oliveira, KRL Freire, R Aparicio, F Coelho - Structure Reports, 2012 - journals.iucr.org
In the title compound, C14H15NO3, the conformation of the double bond was determined to
be E, confirming the result obtained from two-dimensional NMR data. The five-membered …