Rational Modulation of Interface Microenvironment and Design of the Flow Electrolyzer for COx Electroreduction to Alcohol

J Chen, X Peng, Z Li, B Yang, Q Zhang, J Lu… - Advanced …, 2024 - Wiley Online Library
The electrocatalytic reduction of COx (including CO2 and CO) into value‐added fuels and
chemicals, particularly multi‐carbon (C2+) alcohols, presents a significant opportunity to …

Selective and stable CO2 electroreduction at high rates via control of local H2O/CO2 ratio

J Chen, H Qiu, Y Zhao, H Yang, L Fan, Z Liu… - Nature …, 2024 - nature.com
Controlling the concentrations of H2O and CO2 at the reaction interface is crucial for
achieving efficient electrochemical CO2 reduction. However, precise control of these …

Continuously Producing Highly Concentrated and Pure Acetic Acid Aqueous Solution via Direct Electroreduction of CO2

HL Zhu, JR Huang, MD Zhang, C Yu… - Journal of the …, 2024 - ACS Publications
It is crucial to achieve continuous production of highly concentrated and pure C2 chemicals
through the electrochemical CO2 reduction reaction (eCO2RR) for artificial carbon cycling …

Beyond catalysts: enhancing electrocatalytic CO 2 reduction through diverse strategies

L Liu, M Yue, B Li, W **e, N Peng… - Catalysis Science & …, 2024 - pubs.rsc.org
The electrocatalytic CO2 reduction carries extraordinary significance for curbing CO2
emissions while generating value-added chemicals with economic and environmental …

Pathways to reduce the energy cost of carbon monoxide electroreduction to ethylene

T Alkayyali, M Zargartalebi, A Ozden… - Joule, 2024 - cell.com
Summary CO 2-to-CO conversion, followed by CO to value-added products, shows promise
as a high-CO 2 utilization strategy. However, it is necessary to continue to reduce the energy …

Facet-switching of rate-determining step on copper in CO2-to-ethylene electroreduction

YC Zhang, XL Zhang, ZZ Wu, ZZ Niu… - Proceedings of the …, 2024 - National Acad Sciences
Reduction of carbon dioxide (CO2) by renewable electricity to produce multicarbon
chemicals, such as ethylene (C2H4), continues to be a challenge because of insufficient …

Boosting C2+ Alcohols Selectivity and Activity in High‐Current CO Electroreduction using Synergistic Cu/Zn Co‐Catalysts

Z Wu, N Meng, R Yang, M Chen, J Pan… - Angewandte Chemie …, 2024 - Wiley Online Library
The electrosynthesis of multi‐carbon (C2+) alcohols, specifically ethanol and n‐propanol
through CO electroreduction (CORR) in H2O, presents a sustainable pathway for intermittent …

Electrochemical CO2 Activation and Valorization on Metallic Copper and Carbon‐Embedded N‐Coordinated Single Metal MNC Catalysts

X Wang, W Ju, L Liang, M Riyaz, A Bagger… - Angewandte …, 2024 - Wiley Online Library
The electrochemical reductive valorization of CO2, referred to as the CO2RR, is an
emerging approach for the conversion of CO2‐containing feeds into valuable carbonaceous …

Steering the Selectivity of CORR from Acetate to Ethanol via Tailoring the Thermodynamic Activity of Water

J Liu, B Zhang, D Chen, O Peng, H Ma… - Angewandte Chemie …, 2024 - Wiley Online Library
The electrochemical conversion of carbon monoxide (CO) into oxygenated C2+ products at
high rates and selectivity offers a promising approach for the two‐step conversion of carbon …

Field-enhanced CO electroreduction in membrane electrolyzers at a dehydrated interface

W Ren, H Zhang, M Chang, N Chen, W Ma, J Gu, M Lin… - Chem, 2024 - cell.com
Zero-gap membrane electrode assembly (MEA) CO electrolyzer stands as a promising
technology for circular carbon economy. However, current CO electrolyzers are energetically …