Ultrafast electron diffraction: Visualizing dynamic states of matter
Since the discovery of electron-wave duality, electron scattering instrumentation has
developed into a powerful array of techniques for revealing the atomic structure of matter …
developed into a powerful array of techniques for revealing the atomic structure of matter …
Capturing chemistry in action with electrons: realization of atomically resolved reaction dynamics
One of the grand challenges in chemistry has been to directly observe atomic motions
during chemical processes. The depiction of the nuclear configurations in space-time to …
during chemical processes. The depiction of the nuclear configurations in space-time to …
Real-time observation of internal motion within ultrafast dissipative optical soliton molecules
Real-time access to the internal ultrafast dynamics of complex dissipative optical systems
opens new explorations of pulse-pulse interactions and dynamic patterns. We present the …
opens new explorations of pulse-pulse interactions and dynamic patterns. We present the …
Roadmap of ultrafast x-ray atomic and molecular physics
X-ray free-electron lasers (XFELs) and table-top sources of x-rays based upon high
harmonic generation (HHG) have revolutionized the field of ultrafast x-ray atomic and …
harmonic generation (HHG) have revolutionized the field of ultrafast x-ray atomic and …
The photochemical ring-opening of 1, 3-cyclohexadiene imaged by ultrafast electron diffraction
The ultrafast photoinduced ring-opening of 1, 3-cyclohexadiene constitutes a textbook
example of electrocyclic reactions in organic chemistry and a model for photobiological …
example of electrocyclic reactions in organic chemistry and a model for photobiological …
Imaging CF3I conical intersection and photodissociation dynamics with ultrafast electron diffraction
Conical intersections play a critical role in excited-state dynamics of polyatomic molecules
because they govern the reaction pathways of many nonadiabatic processes. However …
because they govern the reaction pathways of many nonadiabatic processes. However …
Ultrafast X-ray scattering reveals vibrational coherence following Rydberg excitation
The coherence and dephasing of vibrational motions of molecules constitute an integral part
of chemical dynamics, influence material properties and underpin schemes to control …
of chemical dynamics, influence material properties and underpin schemes to control …
Self-referenced coherent diffraction x-ray movie of Ångstrom-and femtosecond-scale atomic motion
Time-resolved femtosecond x-ray diffraction patterns from laser-excited molecular iodine are
used to create a movie of intramolecular motion with a temporal and spatial resolution of 30 …
used to create a movie of intramolecular motion with a temporal and spatial resolution of 30 …
Hyperpolarizability and operational magic wavelength in an optical lattice clock
Optical clocks benefit from tight atomic confinement enabling extended interrogation times
as well as Doppler-and recoil-free operation. However, these benefits come at the cost of …
as well as Doppler-and recoil-free operation. However, these benefits come at the cost of …
Different flavors of nonadiabatic molecular dynamics
The Born‐Oppenheimer approximation constitutes a cornerstone of our understanding of
molecules and their reactivity, partly because it introduces a somewhat simplified …
molecules and their reactivity, partly because it introduces a somewhat simplified …