New advances in the use of infrared absorption spectroscopy for the characterization of heterogeneous catalytic reactions

F Zaera - Chemical Society Reviews, 2014 - pubs.rsc.org
Infrared absorption spectroscopy has proven to be one of the most powerful spectroscopic
techniques available for the characterization of catalytic systems. Although the history of IR …

[HTML][HTML] The role of ceria-based nanostructured materials in energy applications

M Melchionna, P Fornasiero - Materials Today, 2014 - Elsevier
Ceria (CeO 2) is enjoying increasing popularity in catalytic applications, and in some cases
has established itself as an irreplaceable component. The reasons for such success stem …

On the structure dependence of CO oxidation over CeO2 nanocrystals with well-defined surface planes

Z Wu, M Li, SH Overbury - Journal of Catalysis, 2012 - Elsevier
CO oxidation is a model reaction for probing the redox property of ceria-based catalysts. In
this study, CO oxidation was investigated over ceria nanocrystals with defined surface …

Gold supported on metal-doped ceria catalysts (M= Zr, Zn and Fe) for the preferential oxidation of CO (PROX)

OH Laguna, FR Sarria, MA Centeno, JA Odriozola - Journal of Catalysis, 2010 - Elsevier
A series of ceria oxides doped with 10mol.% of Zr, Zn and Fe have been prepared by a
pseudo sol–gel method throughout the thermal decomposition of the corresponding metallic …

Quantitative analysis of adsorbate concentrations by diffuse reflectance FT-IR

J Sirita, S Phanichphant, FC Meunier - Analytical chemistry, 2007 - ACS Publications
Fully quantitative analyses of DRIFTS data are required when the surface concentrations
and the specific rate constants of reaction (or desorption) of adsorbates are needed to …

Synergy between Brønsted Acid Sites and Carbonaceous Deposits during Skeletal 1-Butene Isomerization over Ferrierite

KL Hebisch, R Goel, K Gołą̨bek, PA Chmielniak… - ACS …, 2024 - ACS Publications
During skeletal 1-butene isomerization over ferrierite carbonaceous deposits block 98% of
the micropores within 24 h, rendering them effectively inaccessible to reactants, while the …

The design and testing of kinetically-appropriate operando spectroscopic cells for investigating heterogeneous catalytic reactions

FC Meunier - Chemical Society Reviews, 2010 - pubs.rsc.org
This tutorial review discusses some of the current designs of reaction cells used for
operando spectroscopy (X-ray absorption, UV-vis, Raman, transmission FTIR and DRIFTS) …

Influence of crystal size and probe molecule on diffusion in hierarchical ZSM-5 zeolites prepared by desilication

FC Meunier, D Verboekend, JP Gilson… - Microporous and …, 2012 - Elsevier
The improvement of molecular transport properties of hierarchical H-ZSM-5 obtained by
desilication was evidenced by studying the desorption of o-xylene and isooctane by in situ …

Adding diffuse reflectance infrared Fourier transform spectroscopy capability to extended x-ray-absorption fine structure in a new cell to study solid catalysts in …

GL Chiarello, M Nachtegaal, V Marchionni… - Review of Scientific …, 2014 - pubs.aip.org
We describe a novel cell used to combine in situ transmission X-ray absorption
spectroscopy (XAS) with diffuse reflectance infrared Fourier transform spectroscopy …

Assessment of the Reaction Location of Skeletal 1-Butene Isomerization over Ferrierite

PA Chmielniak, KL Hebisch, UP Kim, JC Kenvin… - ACS …, 2024 - ACS Publications
The pore accessibility of fresh and spent ferrierite (FER) during skeletal 1-butene
isomerization is assessed via probe molecule adsorption. Argon and nitrogen adsorption …