Unraveling the structure and dynamics of excitons in semiconductor quantum dots

P Kambhampati - Accounts of chemical research, 2011 - ACS Publications
The quantum dot, one of the central materials in nanoscience, is a semiconductor crystal
with a physical size on the nanometer length scale. It is often called an “artificial atom” …

Synthesis and properties of strongly quantum-confined cesium lead halide perovskite nanocrystals

T Qiao, DH Son - Accounts of Chemical Research, 2021 - ACS Publications
Conspectus Semiconducting metal halide perovskite (MHP) nanocrystals have emerged as
an important new class of materials as the source of photons and charges for various …

Red, green and blue lasing enabled by single-exciton gain in colloidal quantum dot films

C Dang, J Lee, C Breen, JS Steckel… - Nature …, 2012 - nature.com
Colloidal quantum dots exhibit efficient photoluminescence with widely tunable bandgaps
as a result of quantum confinement effects. Such quantum dots are emerging as an …

Hot exciton relaxation dynamics in semiconductor quantum dots: radiationless transitions on the nanoscale

P Kambhampati - The Journal of Physical Chemistry C, 2011 - ACS Publications
The ability to confine electrons and holes in semiconductor quantum dots (QDs) in the form
of excitons creates an electronic structure which is both novel and potentially useful for a …

Ultrafast hole relaxation dynamics in quantum dots revealed by two-dimensional electronic spectroscopy

PJ Brosseau, JJ Geuchies, D Jasrasaria… - Communications …, 2023 - nature.com
Elucidating the population dynamics of correlated electron-hole pairs (bound excitons) in
semiconducting quantum dots (QDs) is key for develo** our fundamental understanding of …

Direct observation of higher multiexciton formation and annihilation in CdSe quantum dots

DP Strandell, A Ghosh, D Zenatti… - The Journal of …, 2023 - ACS Publications
Most experiments on multiexcitons (MX) in quantum dots focused on the biexciton (XX),
which is now well-understood. In contrast, there is little understanding of higher MX in …

Fast Polaron Formation and Low Carrier Mobility in Defect-Free Polyhedral CsPbBr3 Perovskite Nanocrystals

K Justice Babu, G Kaur, A Shukla, R Saha, A Kaur… - ACS …, 2022 - ACS Publications
Albeit enormous achievement has already been made in photovoltaic and optoelectronic
fields with perovskites, further advancement is needed to address key challenges …

Light Emission from CsPbBr3 Metal Halide Perovskite Nanocrystals Arises from Dual Emitting States with Distinct Lattice Couplings

DP Strandell, P Kambhampati - Nano Letters, 2023 - ACS Publications
Metal halide perovskite nanocrystals are under intense investigation for their outstanding
optical and electronic properties. The presence of higher fine structure states, let alone …

Light-induced activation of forbidden exciton transition in strongly confined perovskite quantum dots

D Rossi, H Wang, Y Dong, T Qiao, X Qian, DH Son - ACS nano, 2018 - ACS Publications
We report the strong light-induced activation of forbidden exciton transition in CsPbBr3
perovskite quantum dots mediated by the symmetry-breaking polaron that modifies the …

Nanoparticles, nanocrystals, and quantum dots: What are the implications of size in colloidal nanoscale materials?

P Kambhampati - The Journal of Physical Chemistry Letters, 2021 - ACS Publications
Semiconductor nanoparticles (NP) or nanocrystals (NC) have been investigated for many
decades, with particular acceleration in interest upon the discovery of quantum confinement …