Attosecond spectroscopy for the investigation of ultrafast dynamics in atomic, molecular and solid-state physics

R Borrego-Varillas, M Lucchini… - Reports on Progress in …, 2022 - iopscience.iop.org
Since the first demonstration of the generation of attosecond pulses (1 as= 10− 18 s) in the
extreme-ultraviolet spectral region, several measurement techniques have been introduced …

Advancing time-and angle-resolved photoemission spectroscopy: The role of ultrafast laser development

MX Na, AK Mills, DJ Jones - Physics Reports, 2023 - Elsevier
In the last decade, there has been a proliferation of laser sources for time-and angle-
resolved photoemission spectroscopy (TR-ARPES), building on the proven capability of this …

Snapshots of non-equilibrium Dirac carrier distributions in graphene

I Gierz, JC Petersen, M Mitrano, C Cacho, ICE Turcu… - Nature materials, 2013 - nature.com
The optical properties of graphene are made unique by the linear band structure and the
vanishing density of states at the Dirac point. It has been proposed that even in the absence …

Evidence for topological defects in a photoinduced phase transition

A Zong, A Kogar, YQ Bie, T Rohwer, C Lee, E Baldini… - Nature Physics, 2019 - nature.com
Upon excitation with an intense laser pulse, a symmetry-broken ground state can undergo a
non-equilibrium phase transition through pathways different from those in thermal …

Direct view of hot carrier dynamics in graphene

JC Johannsen, S Ulstrup, F Cilento, A Crepaldi… - Physical Review Letters, 2013 - APS
The ultrafast dynamics of excited carriers in graphene is closely linked to the Dirac spectrum
and plays a central role for many electronic and optoelectronic applications. Harvesting …

Formation of long-lived dark states during electronic relaxation of pyrimidine nucleobases studied using extreme ultraviolet time-resolved photoelectron spectroscopy

Y Miura, Y Yamamoto, S Karashima… - Journal of the …, 2023 - ACS Publications
Ultrafast electronic relaxation of nucleobases from 1ππ* states to the ground state (S0) is
considered essential for the photostability of DNA. However, transient absorption …

Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution

EJ Sie, T Rohwer, C Lee, N Gedik - Nature communications, 2019 - nature.com
High harmonic generation of ultrafast laser pulses can be used to perform angle-resolved
photoemission spectroscopy (ARPES) to map the electronic band structure of materials with …

Highly efficient and aberration-free off-plane grating spectrometer and monochromator for EUV—soft X-ray applications

J Li, K Li, X Zhang, D Popmintchev, H Xu… - Light: Science & …, 2024 - nature.com
We demonstrate a novel flat-field, dual-optic imaging EUV—soft X-ray spectrometer and
monochromator that attains an unprecedented throughput efficiency exceeding 60% by …

Tracking primary thermalization events in graphene with photoemission at extreme time scales

I Gierz, F Calegari, S Aeschlimann… - Physical review …, 2015 - APS
Direct and inverse Auger scattering are amongst the primary processes that mediate the
thermalization of hot carriers in semiconductors. These two processes involve the …

Observation of Ultrafast Free Carrier Dynamics in Single Layer MoS2

A Grubišić Čabo, JA Miwa, SS Grønborg… - Nano …, 2015 - ACS Publications
The dynamics of excited electrons and holes in single layer (SL) MoS2 have so far been
difficult to disentangle from the excitons that dominate the optical response of this material …