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[HTML][HTML] Pursuing excitonic energy transfer with programmable DNA-based optical breadboards
DNA nanotechnology has now enabled the self-assembly of almost any prescribed 3-
dimensional nanoscale structure in large numbers and with high fidelity. These structures …
dimensional nanoscale structure in large numbers and with high fidelity. These structures …
Exciton–vibrational coupling in the dynamics and spectroscopy of Frenkel excitons in molecular aggregates
The influence of exciton–vibrational coupling on the optical and transport properties of
molecular aggregates is an old problem that gained renewed interest in recent years. On the …
molecular aggregates is an old problem that gained renewed interest in recent years. On the …
Non-classicality of the molecular vibrations assisting exciton energy transfer at room temperature
Advancing the debate on quantum effects in light-initiated reactions in biology requires clear
identification of non-classical features that these processes can exhibit and utilize. Here we …
identification of non-classical features that these processes can exhibit and utilize. Here we …
Photonics meets excitonics: natural and artificial molecular aggregates
Organic molecules store the energy of absorbed light in the form of charge-neutral molecular
excitations–Frenkel excitons. Usually, in amorphous organic materials, excitons are viewed …
excitations–Frenkel excitons. Usually, in amorphous organic materials, excitons are viewed …
Ultrafast excitation energy transfer dynamics in photosynthetic pigment–protein complexes
Photosynthetically active membranes of certain bacteria and higher plants contain antenna
systems which surround the reaction center to increase its absorption cross section for the …
systems which surround the reaction center to increase its absorption cross section for the …
A quantum algorithm from response theory: Digital quantum simulation of two-dimensional electronic spectroscopy
Multidimensional optical spectroscopies are powerful techniques to investigate energy
transfer pathways in natural and artificial systems. Because of the high information content of …
transfer pathways in natural and artificial systems. Because of the high information content of …
Exciton delocalization in indolenine squaraine aggregates templated by DNA holliday junction scaffolds
OA Mass, CK Wilson, SK Roy, MS Barclay… - The Journal of …, 2020 - ACS Publications
Exciton delocalization plays a prominent role in the photophysics of molecular aggregates,
ultimately governing their particular function or application. Deoxyribonucleic acid (DNA) is a …
ultimately governing their particular function or application. Deoxyribonucleic acid (DNA) is a …
Pump–probe spectroscopy of dissipative energy transfer dynamics in photosynthetic antenna complexes: A density matrix approach
The photoinduced ultrafast dynamics of singlet excitons in light-harvesting antennae is
investigated using multilevel Redfield theory. Formulating the equations of motion for the …
investigated using multilevel Redfield theory. Formulating the equations of motion for the …
Large Davydov splitting and strong fluorescence suppression: an investigation of exciton delocalization in DNA-templated Holliday junction dye aggregates
Exciton delocalization in dye aggregate systems is a phenomenon that is revealed by
spectral features, such as Davydov splitting, J-and H-aggregate behavior, and fluorescence …
spectral features, such as Davydov splitting, J-and H-aggregate behavior, and fluorescence …
Multi-layer multi-configuration time-dependent Hartree (ML-MCTDH) approach to the correlated exciton-vibrational dynamics in the FMO complex
The coupled quantum dynamics of excitonic and vibrational degrees of freedom is
investigated for high-dimensional models of the Fenna-Matthews-Olson complex. This …
investigated for high-dimensional models of the Fenna-Matthews-Olson complex. This …