From glycals to aminosugars: a challenging test for new stereoselective aminohydroxylation and related methodologies

S Mirabella, F Cardona, A Goti - Organic & Biomolecular Chemistry, 2016 - pubs.rsc.org
The introduction of amino functionalities in a regio-and stereoselective manner onto sugar
scaffolds represents a great challenge in carbohydrate synthesis. The most relevant …

Site selective gold (I)-catalysed benzylic C–H amination via an intermolecular hydride transfer to triazolinediones

K Bevernaege, NV Tzouras, A Poater, L Cavallo… - Chemical …, 2023 - pubs.rsc.org
Triazolinediones are known as highly reactive dienophiles that can also act as electrophilic
amination reagents towards enolisable C–H bonds (ionic pathway) or weak C–H bonds …

Nickel-Catalyzed Dearomative trans-1,2-Carboamination

LW Hernandez, U Klöckner, J Pospech… - Journal of the …, 2018 - ACS Publications
We describe the development of an arenophile-mediated, nickel-catalyzed dearomative
trans-1, 2-carboamination protocol. A range of readily available aromatic compounds was …

Palladium-Catalyzed Dearomative syn-1,4-Carboamination

M Okumura, AS Shved, D Sarlah - Journal of the American …, 2017 - ACS Publications
A dearomative 1, 4-carboamination of arenes has been achieved using arenophile
cycloaddition and subsequent palladium-catalyzed substitution with nonstabilized lithium …

Diels–Alder and ene reactions of singlet oxygen, nitroso compounds and triazolinediones: transition states and mechanisms from contemporary theory

AG Leach, KN Houk - Chemical communications, 2002 - pubs.rsc.org
Singlet oxygen, nitroso compounds and triazolinediones have similar electronic structures:
they share a low lying LUMO, making them powerful electrophiles, and a high lying HOMO …

Palladium-Catalyzed Dearomative syn-1,4-Diamination

WC Wertjes, M Okumura, D Sarlah - Journal of the American …, 2018 - ACS Publications
Herein we report a dearomative syn-1, 4-diamination protocol using simple nonactivated
arenes and amines. This one-pot method utilizes arene–arenophile para-cycloadducts …

Palladium‐Catalyzed Dearomative syn‐1,4‐Carboamination with Grignard Reagents

C Tang, M Okumura, Y Zhu, AR Hooper… - Angewandte …, 2019 - Wiley Online Library
A protocol for palladium‐catalyzed dearomative functionalization of simple, nonactivated
arenes with Grignard reagents has been established. This one‐pot method features a visible …

Arenophile-mediated dearomative functionalization strategies

M Okumura, D Sarlah - Synlett, 2018 - thieme-connect.com
The dearomatization of arenes is a fundamental synthetic strategy, providing a direct
connection between simple hydrocarbons and valuable, more complex intermediates. While …

Dynamic Covalent Chemistry: A Facile Room‐Temperature, Reversible, Diels–Alder Reaction between Anthracene Derivatives and N‐Phenyltriazolinedione

N Roy, JM Lehn - Chemistry–An Asian Journal, 2011 - Wiley Online Library
A series of readily accessible, dynamic Diels–Alder reactions that are reversible at room
temperature have been developed between anthracene derivatives as dienes and N‐phenyl …

Synthesis of Carbamates from Diethoxycarbonyl Hydrazine Derivatives by E1cB Eliminative Cleavage of the N−N′-Bond Rather than Reduction

P Magnus, N Garizi, KA Seibert, A Ornholt - Organic Letters, 2009 - ACS Publications
Synthesis of Carbamates from Diethoxycarbonyl Hydrazine Derivatives by E1cB Eliminative
Cleavage of the N−N′-Bond Rather than Reduction | Organic Letters ACS ACS Publications …