Time-resolved experiments on gas-phase atoms and molecules with XUV and X-ray free-electron lasers

D Rolles - Advances in Physics: X, 2023 - Taylor & Francis
Over the last 20 years, XUV and X-ray free-electron lasers have enabled a wide variety of
time-resolved experiments that have dramatically advanced our understanding of ultrafast …

Attosecond coherent electron motion in Auger-Meitner decay

S Li, T Driver, P Rosenberger, EG Champenois, J Duris… - Science, 2022 - science.org
In quantum systems, coherent superpositions of electronic states evolve on ultrafast time
scales (few femtoseconds to attoseconds; 1 attosecond= 0.001 femtoseconds= 10− 18 …

Attosecond spectroscopy for filming the ultrafast movies of atoms, molecules and solids

L He, X Zhu, W Cao, P Lan, P Lu - Chinese Physics B, 2022 - iopscience.iop.org
Three decades ago, a highly nonlinear nonpertubative phenomenon, now well-known as
the high harmonic generation (HHG), was discovered when intense laser irradiates gaseous …

Correlation-driven transient hole dynamics resolved in space and time in the isopropanol molecule

T Barillot, O Alexander, B Cooper, T Driver, D Garratt… - Physical Review X, 2021 - APS
The possibility of suddenly ionized molecules undergoing extremely fast electron hole (or
hole) dynamics prior to significant structural change was first recognized more than 20 years …

Simultaneous monitoring of mitochondrial viscosity and membrane potential based on fluorescence changing and location switching of carbon dots in living cells

S Guo, Y Sun, Z Wu, R Yang, L Qu, Z Li - Carbon, 2022 - Elsevier
Highlights•The fluorescence of Carbon Dots (CDs) was specifically turned on as the
viscosity of solvents increased.•Fluctuation of mitochondrial membrane potential was …

Accurate core excitation and ionization energies from a state-specific coupled-cluster singles and doubles approach

JE Arias-Martinez, LA Cunha, KJ Oosterbaan… - Physical Chemistry …, 2022 - pubs.rsc.org
We investigate the use of orbital-optimized references in conjunction with single-reference
coupled-cluster theory with single and double substitutions (CCSD) for the study of core …

Probing resonant photoionization time delay by self-referenced molecular attoclock

J Tong, X Liu, W Dong, W Jiang, M Zhu, Y Xu, Z Zuo… - Physical Review Letters, 2022 - APS
Attosecond time-resolved electron tunneling dynamics have been investigated by using
attosecond angular streaking spectroscopy, where a clock reference to the laser field vector …

Probing Electronic Coherence between Core-Level Vacancies at Different Atomic Sites

J Wang, T Driver, PL Franz, P Kolorenč, E Thierstein… - Physical Review X, 2025 - APS
The detailed understanding of electronic coherence in quantum systems requires
measurements on the attosecond timescale. Attosecond x-ray pulses enable the study of …

Auger–Meitner and x-ray absorption spectra of ethylene cation: insight into conical intersection dynamics

BN Cabral Tenorio, J Pedersen, M Barbatti… - The Journal of …, 2023 - ACS Publications
We present a theoretical investigation of the near-edge X-ray absorption fine structure and
the Auger–Meitner decay spectra of ethylene and its cation. Herein, we demonstrate that our …

Ultrafast condensed matter physics at attoseconds

SQ Hu, S Meng - Chinese Physics Letters, 2023 - iopscience.iop.org
Our understanding of how photons couple to different degrees of freedom in solids forms the
bedrock of ultrafast physics and materials sciences. In this review, the emergent ultrafast …