The acidity of atmospheric particles and clouds

HOT Pye, A Nenes, B Alexander, AP Ault… - Atmospheric …, 2020 - acp.copernicus.org
Acidity, defined as pH, is a central component of aqueous chemistry. In the atmosphere, the
acidity of condensed phases (aerosol particles, cloud water, and fog droplets) governs the …

Multiphase oxidation of sulfur dioxide in aerosol particles: Implications for sulfate formation in polluted environments

T Liu, AWH Chan, JPD Abbatt - Environmental Science & …, 2021 - ACS Publications
Atmospheric oxidation of sulfur dioxide (SO2) forms sulfate-containing aerosol particles that
impact air quality, climate, and human and ecosystem health. It is well-known that in-cloud …

[HTML][HTML] Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds

A Tilgner, T Schaefer, B Alexander… - Atmospheric …, 2021 - acp.copernicus.org
The acidity of aqueous atmospheric solutions is a key parameter driving both the partitioning
of semi-volatile acidic and basic trace gases and their aqueous-phase chemistry. In addition …

[HTML][HTML] Heterogeneous sulfate aerosol formation mechanisms during wintertime Chinese haze events: air quality model assessment using observations of sulfate …

J Shao, Q Chen, Y Wang, X Lu, P He… - Atmospheric …, 2019 - acp.copernicus.org
Air quality models have not been able to reproduce the magnitude of the observed
concentrations of fine particulate matter (PM 2.5) during wintertime Chinese haze events …

[HTML][HTML] DMS oxidation and sulfur aerosol formation in the marine troposphere: a focus on reactive halogen and multiphase chemistry

Q Chen, T Sherwen, M Evans… - … Chemistry and Physics, 2018 - acp.copernicus.org
The oxidation of dimethyl sulfide (DMS) in the troposphere and subsequent chemical
conversion into sulfur dioxide (SO 2) and methane sulfonic acid (MSA) are key processes for …

Atmospheric Δ17O(NO3) reveals nocturnal chemistry dominates nitrate production in Bei**g haze

P He, Z **e, X Chi, X Yu, S Fan, H Kang… - Atmospheric …, 2018 - acp.copernicus.org
The rapid mass increase of atmospheric nitrate is a critical driving force for the occurrence of
fine-particle pollution (referred to as haze hereafter) in Bei**g. However, the exact …

Isotopic constraints on heterogeneous sulfate production in Bei**g haze

P He, B Alexander, L Geng, X Chi, S Fan… - Atmospheric …, 2018 - acp.copernicus.org
Discerning mechanisms of sulfate formation during fine-particle pollution (referred to as
haze hereafter) in Bei**g is important for understanding the rapid evolution of haze and for …

Sulfate production by reactive bromine: Implications for the global sulfur and reactive bromine budgets

Q Chen, JA Schmidt, V Shah, L Jaeglé… - Geophysical …, 2017 - Wiley Online Library
Sulfur and reactive bromine (Br y) play important roles in tropospheric chemistry and the
global radiation budget. The oxidation of dissolved SO2 (S (IV)) by HOBr increases sulfate …

Isotopic evidence for acidity-driven enhancement of sulfate formation after SO2 emission control

S Hattori, Y Iizuka, B Alexander, S Ishino, K Fujita… - Science …, 2021 - science.org
After the 1980s, atmospheric sulfate reduction is slower than the dramatic reductions in
sulfur dioxide (SO2) emissions. However, a lack of observational evidence has hindered the …

The sensitivity of Southern Ocean aerosols and cloud microphysics to sea spray and sulfate aerosol production in the HadGEM3-GA7. 1 chemistry–climate model

LE Revell, S Kremser, S Hartery… - Atmospheric …, 2019 - acp.copernicus.org
With low concentrations of tropospheric aerosol, the Southern Ocean offers a “natural
laboratory” for studies of aerosol–cloud interactions. Aerosols over the Southern Ocean are …