Explicitly correlated electrons in molecules

C Hattig, W Klopper, A Kohn, DP Tew - Chemical reviews, 2012 - ACS Publications
One of the central challenges of computational molecular investigation is the solution of the
time-independent, nonrelativistic BornÀ Oppenheimer electronic Schrödinger equation. For …

Computing vibrational spectra from ab initio molecular dynamics

M Thomas, M Brehm, R Fligg, P Vöhringer… - Physical Chemistry …, 2013 - pubs.rsc.org
We review several methods for the calculation of vibrational spectra from ab initio molecular
dynamics (AIMD) simulations and we present a new implementation in the trajectory …

Simplified CCSD (T)-F12 methods: Theory and benchmarks

G Knizia, TB Adler, HJ Werner - The Journal of chemical physics, 2009 - pubs.aip.org
The simple and efficient CCSD (T)-F 12 x approximations (x= a, b) we proposed in a recent
communication [TB Adler, G. Knizia, and H.-J. Werner, J. Chem. Phys. 127, 221106 (2007)] …

Chemical accuracy in ab initio thermochemistry and spectroscopy: current strategies and future challenges

KA Peterson, D Feller, DA Dixon - Theoretical Chemistry Accounts, 2012 - Springer
The current state of the art in wavefunction-based electronic structure methods is illustrated
via discussions of the most important effects incorporated into a selection of high-accuracy …

On the effectiveness of CCSD (T) complete basis set extrapolations for atomization energies

D Feller, KA Peterson, J Grant Hill - The Journal of chemical physics, 2011 - pubs.aip.org
The leading cause of error in standard coupled cluster theory calculations of thermodynamic
properties such as atomization energies and heats of formation originates with the truncation …

Harmonic and anharmonic vibrational frequency calculations with the double-hybrid B2PLYP method: analytic second derivatives and benchmark studies

M Biczysko, P Panek, G Scalmani… - Journal of Chemical …, 2010 - ACS Publications
This work aims to provide reliable benchmark data on the accuracy of harmonic and
anharmonic vibrational frequencies computed with the B2PLYP double-hybrid density …

Explicitly correlated multireference configuration interaction: MRCI-F12

T Shiozaki, G Knizia, HJ Werner - The Journal of chemical physics, 2011 - pubs.aip.org
An internally contracted multireference configuration interaction is developed which employs
wave functions that explicitly depend on the electron–electron distance (MRCI-F12). This …

Explicitly correlated coupled cluster methods with pair-specific geminals

HJ Werner, G Knizia, FR Manby - Molecular Physics, 2011 - Taylor & Francis
Explicitly correlated MP2-F12 and CCSD (T)-F12 methods with orbital-pair-specific Slater-
type geminals are proposed. The fixed amplitude ansatz of Ten-no is used, and different …

Further benchmarks of a composite, convergent, statistically calibrated coupled-cluster-based approach for thermochemical and spectroscopic studies

D Feller, KA Peterson, DA Dixon - Molecular Physics, 2012 - Taylor & Francis
A flexible, high-level, composite approach based on coupled cluster theory has been used
to predict the atomization energies and equilibrium structures of 13 small, first-row …

Optimized complementary auxiliary basis sets for explicitly correlated methods: aug-cc-pVnZ orbital basis sets

KE Yousaf, KA Peterson - Chemical Physics Letters, 2009 - Elsevier
Compact auxiliary basis sets matched to the standard aug-cc-pVnZ and aug-cc-pV (n+ d) Z
orbital basis sets have been developed for use as resolution-of-the-identity (RI) sets in …