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The oxygen evolution reaction drives passivity breakdown for Ni–Cr–Mo alloys
Corrosion is the main factor limiting the lifetime of metallic materials, and a fundamental
understanding of the governing mechanism and surface processes is difficult to achieve …
understanding of the governing mechanism and surface processes is difficult to achieve …
Unsupervised analysis of optical imaging data for the discovery of reactivity patterns in metal alloy
Operando wide‐field optical microscopy imaging yields a wealth of information about the
reactivity of metal interfaces, yet the data are often unstructured and challenging to process …
reactivity of metal interfaces, yet the data are often unstructured and challenging to process …
Imaging Gas-Phase Methyl Radicals over a Ag/SiO2 Catalyst during the Partial Oxidation of Methanol
We report the operando imaging of the methyl radical mole fraction above a working
catalyst. Using photofragmentation laser-induced fluorescence (PF-LIF), we imaged methyl …
catalyst. Using photofragmentation laser-induced fluorescence (PF-LIF), we imaged methyl …
[HTML][HTML] Ambient pressure operando catalytic characterization by combining PM-IRRAS with planar laser-induced fluorescence and surface optical reflectance …
We present a combination of optical operando techniques that allow us to bridge the
pressure gap in heterogeneous catalysis. By combining Polarization Modulated-InfraRed …
pressure gap in heterogeneous catalysis. By combining Polarization Modulated-InfraRed …
Constraining reaction pathways for methanol oxidation through operando interrogation of both the surface and the near-surface gas phase
We combine near-surface molecular beam mass spectrometry—a probe of the gas phase
within hundreds of micrometers of catalyst surfaces—and surface-sensitive infrared …
within hundreds of micrometers of catalyst surfaces—and surface-sensitive infrared …
A polycrystalline Pd surface studied by two-dimensional surface optical reflectance during CO oxidation: Bridging the materials gap
Industrial catalysts are complex materials systems operating in harsh environments. The
active parts of the catalysts are nanoparticles that expose different facets with different …
active parts of the catalysts are nanoparticles that expose different facets with different …
Magnetic field-assisted nanochain formation of intermixed catalytic Co–Pd nanoparticles
Engineering on the nanoscale often involves optimizing performance by designing and
creating new types of nanostructured materials. Multifunctional nanoparticles can be formed …
creating new types of nanostructured materials. Multifunctional nanoparticles can be formed …
[HTML][HTML] Multi modal time-resolved infrared and X-ray spectroscopic operando studies of the CO oxidation and NO reduction reactions on Rh (111)
We present an operando study where Ambient-Pressure X-ray Photoelectron Spectroscopy
(AP-XPS), Polarization Modulation-InfraRed Reflection Absorption Spectroscopy (PM …
(AP-XPS), Polarization Modulation-InfraRed Reflection Absorption Spectroscopy (PM …
[HTML][HTML] Velocity-selected spatial map ion imaging spectrometer for direct imaging of near-surface catalytic activity
We propose and demonstrate an approach permitting direct imaging of the spatial
distribution of gas-surface reaction products with< 60 μm lateral spatial resolution using a …
distribution of gas-surface reaction products with< 60 μm lateral spatial resolution using a …
Temperature dependent collisional quenching rates of CH (A) by methanol, acetone, methane, oxygen, and nitrogen
Laser-induced fluorescence is a widely used technique for measuring the concentrations of
gaseous species in reactive environments. To determine absolute number densities from …
gaseous species in reactive environments. To determine absolute number densities from …