Interstellar anions: the role of quantum chemistry

RC Fortenberry - The Journal of Physical Chemistry A, 2015‏ - ACS Publications
Six anions have been conclusively detected in the interstellar medium (ISM). They all arrived
within a five-year window ending five years ago. Why have no new anions been detected? It …

Photodetachment as a destruction mechanism for CN− and C3N− anions in circumstellar envelopes

SS Kumar, D Hauser, R **dra, T Best… - The Astrophysical …, 2013‏ - iopscience.iop.org
Absolute photodetachment cross sections of two anions of astrophysical importance CN−
and C 3 N− were measured to be (1.18±(0.03) stat (0.17) sys)× 10− 17 cm 2 and …

Formation of , , and Molecules by Radiative Electron Attachment and their Destruction by Photodetachment

M Khamesian, N Douguet, S Fonseca dos Santos… - Physical review …, 2016‏ - APS
The existence of negative ions in interstellar clouds has been associated for several
decades with the process of radiative electron attachment. In this Letter, we report …

Theoretical prediction of new dipole-bound singlet states for anions of interstellar interest

RC Fortenberry, TD Crawford - The Journal of chemical physics, 2011‏ - pubs.aip.org
Anions that exhibit dipole-bound singlet states have been proposed as a potential class of
molecules that may be identified in the interstellar medium. Using high-level coupled cluster …

Vibrational Predissociation Spectra of C2N and C3N: Bending and Stretching Vibrations

F Dahlmann, DF Dinu, P Jusko, C Lochmann… - …, 2023‏ - Wiley Online Library
We present infrared predissociation spectra of C2N−(H2) and C 3N−(H2) in the 300–1850
cm− 1 range. Measurements were performed using the FELion cryogenic ion trap end user …

Bound and continuum-embedded states of cyanopolyyne anions

W Skomorowski, S Gulania, AI Krylov - Physical Chemistry Chemical …, 2018‏ - pubs.rsc.org
Cyanopolyyne anions were among the first anions discovered in the interstellar medium.
The discovery has raised questions about the routes of formation of these anions in space …

The role of internal photons on the chemistry of the circumstellar envelopes of AGB stars

M Van de Sande, TJ Millar - The Astrophysical Journal, 2019‏ - iopscience.iop.org
Recent high spatial resolution observations of gas and dust in the circumstellar envelopes
(CSEs) of AGB stars indicate morphologies much more complex than the smooth density …

Influence of a Supercritical Electric Dipole Moment on the Photodetachment of

M Simpson, M Nötzold, T Michaelsen, R Wild… - Physical Review Letters, 2021‏ - APS
Threshold photodetachment spectroscopy of the molecular ion C 3 N-has been performed at
both 16 (1) and 295 (2) K in a 22-pole ion trap. The 295 (2) K spectrum shows a large …

Low temperature reaction kinetics of CN−+ HC3N and implications for the growth of anions in Titan's atmosphere

L Biennier, S Carles, D Cordier, JC Guillemin… - Icarus, 2014‏ - Elsevier
Abstract The Cassini–Huygens probe has uncovered the existence of a profusion of
negatively charged molecular species in the upper atmosphere of Titan (∼ 950 km). The …

Additional diffuse functions in basis sets for dipole-bound excited states of anions

WJ Morgan, RC Fortenberry - Theoretical Chemistry Accounts, 2015‏ - Springer
The existence of dipole-bound excited states has largely been shown by previous
computation through the use of the standard LCAO-MO creation with numerous and diffuse …