Time-resolved ARPES studies of quantum materials

F Boschini, M Zonno, A Damascelli - Reviews of Modern Physics, 2024 - APS
Angle-resolved photoemission spectroscopy (ARPES), with its exceptional sensitivity to both
the binding energy and the momentum of valence electrons in solids, provides unparalleled …

Directly visualizing the momentum-forbidden dark excitons and their dynamics in atomically thin semiconductors

J Madéo, MKL Man, C Sahoo, M Campbell, V Pareek… - Science, 2020 - science.org
Resolving momentum degrees of freedom of excitons, which are electron-hole pairs bound
by the Coulomb attraction in a photoexcited semiconductor, has remained an elusive goal …

Hot electron relaxation dynamics in semiconductors: assessing the strength of the electron–phonon coupling from the theoretical and experimental viewpoints

J Sjakste, K Tanimura, G Barbarino… - Journal of Physics …, 2018 - iopscience.iop.org
The rapid development of the computational methods based on density functional theory, on
the one hand, and of time-, energy-, and momentum-resolved spectroscopy, on the other …

Experimental measurement of the intrinsic excitonic wave function

MKL Man, J Madéo, C Sahoo, K **e, M Campbell… - Science …, 2021 - science.org
An exciton, a two-body composite quasiparticle formed of an electron and hole, is a
fundamental optical excitation in condensed matter systems. Since its discovery nearly a …

Momentum-Resolved Observation of Exciton Formation Dynamics in Monolayer WS2

R Wallauer, R Perea-Causin, L Münster, S Zajusch… - Nano …, 2021 - ACS Publications
The dynamics of momentum-dark exciton formation in transition metal dichalcogenides is
difficult to measure experimentally, as many momentum-indirect exciton states are not …

Direct measurement of key exciton properties: Energy, dynamics, and spatial distribution of the wave function

S Dong, M Puppin, T Pincelli, S Beaulieu… - Natural …, 2021 - Wiley Online Library
Excitons, Coulomb‐bound electron–hole pairs, are the fundamental excitations governing
the optoelectronic properties of semiconductors. Although optical signatures of excitons …

Time-domain observation of interlayer exciton formation and thermalization in a MoSe2/WSe2 heterostructure

VR Policht, H Mittenzwey, O Dogadov, M Katzer… - Nature …, 2023 - nature.com
Vertical heterostructures of transition metal dichalcogenides (TMDs) host interlayer excitons
with electrons and holes residing in different layers. With respect to their intralayer …

Ab Initio Calculations of Ultrashort Carrier Dynamics in Two-Dimensional Materials: Valley Depolarization in Single-Layer WSe2

A Molina-Sánchez, D Sangalli, L Wirtz, A Marini - Nano letters, 2017 - ACS Publications
In single-layer WSe2, a paradigmatic semiconducting transition metal dichalcogenide, a
circularly polarized laser field can selectively excite electronic transitions in one of the …

Theory of exciton dynamics in time-resolved ARPES: Intra-and intervalley scattering in two-dimensional semiconductors

D Christiansen, M Selig, E Malic, R Ernstorfer, A Knorr - Physical Review B, 2019 - APS
Time-and angle-resolved photoemission spectroscopy (trARPES) is a powerful
spectroscopic method to measure the ultrafast electron dynamics directly in momentum …

First-principles ultrafast exciton dynamics and time-domain spectroscopies: Dark-exciton mediated valley depolarization in monolayer

HY Chen, D Sangalli, M Bernardi - Physical Review Research, 2022 - APS
Calculations combining first-principles electron-phonon (e-ph) interactions with the
Boltzmann equation enable studies of ultrafast carrier and phonon dynamics. However, in …