Recent Advances in First‐Row Transition‐Metal‐Mediated C− H Halogenation of (Hetero) arenes and Alkanes

A Paik, S Paul, S Bhowmik, R Das… - Asian Journal of …, 2022 - Wiley Online Library
The ubiquity of carbon halogen bonds in the structural core of numerous biomolecules and
pharmaceuticals along with their role as synthetic precursors in various organic reactions …

Inspiration from Nature: influence of engineered ligand scaffolds and auxiliary factors on the reactivity of biomimetic oxidants

G Mukherjee, JK Satpathy, UK Bagha… - ACS …, 2021 - ACS Publications
Enzymes are highly efficient catalysts in Nature that often react with high stereo-, chemo-,
and regioselectivity. Usually, enzymes achieve this selectivity through substrate binding and …

Experimental and theoretical investigation of the tuning of electronic structure in SnO 2 via Co do** for enhanced styrene epoxidation catalysis

J Liu, X Ji, J Shi, L Wang, P Jian, X Yan… - Catalysis Science & …, 2022 - pubs.rsc.org
Exploiting new heterogeneous catalysts composed of earth-abundant elements for various
organic transformations under moderate reaction conditions is of vital importance in modern …

Carbamoyl manganese complexes for epoxidation of alkenes and cycloaddition of epoxides to carbon dioxide

H Hu, Y Li, Y Li, Y Ding, Y Sun, Y Li - Journal of Catalysis, 2023 - Elsevier
There is no precedent for the usage of transition metal carbamoyl complexes (typical
hydrogenase models) as pre-catalysts for oxidation or CO 2 utilization purposes. In this …

Advances in the synthesis and applications of macrocyclic polyamines

Y Gao, L Guo, X Liu, N Chen… - Royal Society Open …, 2024 - royalsocietypublishing.org
Macrocyclic polyamines constitute a significant class of macrocyclic compounds that play a
pivotal role in the realm of supramolecular chemistry. They find extensive applications …

Theoretical exploration on structures, bonding aspects and molecular docking of α-aminophosphonate ligated copper complexes against SARS-CoV-2 proteases

O Yadav, M Kumar, H Mittal, K Yadav… - Frontiers in …, 2022 - frontiersin.org
Recent years have witnessed a growing interest in the biological activity of metal complexes
of α-aminophosphonates. Here for the first time, a detailed DFT study on five α …

Comparative oxidative ability of mononuclear and dinuclear high-valent iron–oxo species towards the activation of methane: does the axial/bridge atom modulate the …

M Ansari, G Rajaraman - Dalton Transactions, 2023 - pubs.rsc.org
Over the years, mononuclear FeIVO species have been extensively studied, but the
presence of dinuclear FeIVO species in soluble methane monooxygenase (sMMO) has …

Effect of Redox-Active Quinoline on the Reactivity and Mechanism of Hydrogen Evolution Reaction (HER) with Pentadentate Polypyridyl-Quinolyl Ligand-Coordinated …

A Paik, C Das, S Paul, A Biswas, S Mehta… - ACS …, 2024 - ACS Publications
Herein, we have introduced a redox-active quinoline moiety in a pentadentate pyridine-
containing N4Py ligand resulting in two quinolines and two pyridines containing 2PyN2Q …

A tale of two topological isomers: Uptuning [FeIV(O)(Me4cyclam)]2+ for olefin epoxidation

B Chandra, F Ahsan, Y Sheng… - Proceedings of the …, 2024 - National Acad Sciences
TMC-anti and TMC-syn, the two topological isomers of [FeIV (O)(TMC)(CH3CN)] 2+(TMC= 1,
4, 8, 11-tetramethyl-1, 4, 8, 11-tetraazacyclotetradecane, or Me4cyclam), differ in the …

Speciation Differences in the Surface Oxidizing Species on FeS2 and NiS2: Reactivity in Hydrogen Atom Transfer and Oxygen Atom Transfer

XB Zhang, H Tian, SH Wu, Y Liu… - ACS Earth and Space …, 2023 - ACS Publications
As the most abundant metal sulfide on Earth's surface, pyrite (FeS2) plays important roles in
the transformation of various elements and contaminants. Noteworthily, pyrite-type metal …