Molecular magnetism, quo vadis? A historical perspective from a coordination chemist viewpoint☆

J Ferrando-Soria, J Vallejo, M Castellano… - Coordination Chemistry …, 2017 - Elsevier
Molecular magnetism has travelled a long way from the pioneering studies on electron
exchange and double exchange or spin crossover and valence tautomerism in small …

Spin states, vibrations and spin relaxation in molecular nanomagnets and spin qubits: a critical perspective

L Escalera-Moreno, JJ Baldoví, A Gaita-Arino… - Chemical …, 2018 - pubs.rsc.org
Very recently the closely related fields of molecular spin qubits, single ion magnets and
single atom magnets have been shaken by unexpected results. We have witnessed a jump …

Coherence in Chemistry: Foundations and Frontiers

JD Schultz, JL Yuly, EA Arsenault, K Parker… - Chemical …, 2024 - ACS Publications
Coherence refers to correlations in waves. Because matter has a wave-particle nature, it is
unsurprising that coherence has deep connections with the most contemporary issues in …

Room temperature quantum coherence in a potential molecular qubit

K Bader, D Dengler, S Lenz, B Endeward… - Nature …, 2014 - nature.com
The successful development of a quantum computer would change the world, and current
internet encryption methods would cease to function. However, no working quantum …

Determining key local vibrations in the relaxation of molecular spin qubits and single-molecule magnets

L Escalera-Moreno, N Suaud… - The journal of …, 2017 - ACS Publications
To design molecular spin qubits and nanomagnets operating at high temperatures, there is
an urgent need to understand the relationship between vibrations and spin relaxation …

A reaction-coordinate perspective of magnetic relaxation

CE Jackson, IP Moseley, R Martinez, S Sung… - Chemical Society …, 2021 - pubs.rsc.org
Understanding and utilizing the dynamic quantum properties of metal ions is the frontier of
many next generation technologies. One property in particular, magnetic relaxation, is a …

Long coherence times in nuclear spin-free vanadyl qubits

CJ Yu, MJ Graham, JM Zadrozny, J Niklas… - Journal of the …, 2016 - ACS Publications
Quantum information processing (QIP) offers the potential to create new frontiers in fields
ranging from quantum biology to cryptography. Two key figures of merit for electronic spin …

Forging solid-state qubit design principles in a molecular furnace

MJ Graham, JM Zadrozny, MS Fataftah… - Chemistry of …, 2017 - ACS Publications
The realization of quantum information processing would disrupt the status quo in the realm
of computation; the extraordinary power of a hypothetical quantum computer motivates …

Spin dynamics and low energy vibrations: insights from vanadyl-based potential molecular qubits

M Atzori, L Tesi, S Benci, A Lunghi… - Journal of the …, 2017 - ACS Publications
Here we report the investigation of the magnetization dynamics of a vanadyl complex with
diethyldithiocarbamate (Et2dtc–) ligands, namely [VO (Et2dtc) 2](1), in both solid-state and …

Chemical control of spin–lattice relaxation to discover a room temperature molecular qubit

MJ Amdur, KR Mullin, MJ Waters, D Puggioni… - Chemical …, 2022 - pubs.rsc.org
The second quantum revolution harnesses exquisite quantum control for a slate of diverse
applications including sensing, communication, and computation. Of the many candidates …