Configurational entropy of glass-forming liquids
The configurational entropy is one of the most important thermodynamic quantities
characterizing supercooled liquids approaching the glass transition. Despite decades of …
characterizing supercooled liquids approaching the glass transition. Despite decades of …
Visualizing slow internal relaxations in a two-dimensional glassy system
Unlike a crystal, a glassy solid state displays slow internal relaxation processes besides
vibrational modes even when structural (α) relaxation is frozen. The precise nature of such …
vibrational modes even when structural (α) relaxation is frozen. The precise nature of such …
Glasses and aging, A statistical mechanics perspective on
We start with a few concise definitions of the most important concepts discussed in this entry.
Glass transition For molecular liquids, the glass transition denotes a crossover from a …
Glass transition For molecular liquids, the glass transition denotes a crossover from a …
Elastic interactions of plastic events in strained amorphous solids before yield
It has been widely accepted that the plastic events of amorphous solids after mechanical
yield belong to a highly correlated avalanche state. However, whether the plastic events …
yield belong to a highly correlated avalanche state. However, whether the plastic events …
Reaching the ideal glass in polymer spheres: Thermodynamics and vibrational density of states
The existence of an ideal glass and the resolution to the Kauzmann paradox is a long-
standing open question in materials science. To address this problem, we exploit the ability …
standing open question in materials science. To address this problem, we exploit the ability …
Atomistic structural mechanism for the glass transition: Entropic contribution
A popular Adam-Gibbs scenario has suggested that the excess entropy of glass and liquid
over crystal dominates the dynamical arrest at the glass transition with exclusive contribution …
over crystal dominates the dynamical arrest at the glass transition with exclusive contribution …
Creating bulk ultrastable glasses by random particle bonding
A recent breakthrough in glass science has been the synthesis of ultrastable glasses via
physical vapor deposition techniques. These samples display enhanced thermodynamic …
physical vapor deposition techniques. These samples display enhanced thermodynamic …
Exploring the soft pinning effect in the dynamics and the structure–dynamics correlation in multicomponent supercooled liquids
We study multicomponent liquids by increasing the mass of 15% of the particles in a binary
Kob–Andersen model. We find that the heavy particles have dual effects on the lighter …
Kob–Andersen model. We find that the heavy particles have dual effects on the lighter …
Configurational entropy of polydisperse supercooled liquids
We propose a computational method to measure the configurational entropy in generic
polydisperse glass-formers. In particular, our method resolves issues related to the diverging …
polydisperse glass-formers. In particular, our method resolves issues related to the diverging …
Computer simulations of the glass transition and glassy materials
We provide an overview of the different types of computational techniques developed over
the years to study supercooled liquids, glassy materials and the physics of the glass …
the years to study supercooled liquids, glassy materials and the physics of the glass …