Configurational entropy of glass-forming liquids

L Berthier, M Ozawa, C Scalliet - The Journal of chemical physics, 2019 - pubs.aip.org
The configurational entropy is one of the most important thermodynamic quantities
characterizing supercooled liquids approaching the glass transition. Despite decades of …

Visualizing slow internal relaxations in a two-dimensional glassy system

Y Chen, Z Ye, K Wang, J Huang, H Tong, Y **… - Nature Physics, 2023 - nature.com
Unlike a crystal, a glassy solid state displays slow internal relaxation processes besides
vibrational modes even when structural (α) relaxation is frozen. The precise nature of such …

Glasses and aging, A statistical mechanics perspective on

F Arceri, FP Landes, L Berthier, G Biroli - Statistical and Nonlinear Physics, 2022 - Springer
We start with a few concise definitions of the most important concepts discussed in this entry.
Glass transition For molecular liquids, the glass transition denotes a crossover from a …

Elastic interactions of plastic events in strained amorphous solids before yield

J Duan, YJ Wang, LH Dai, MQ Jiang - Physical Review Materials, 2023 - APS
It has been widely accepted that the plastic events of amorphous solids after mechanical
yield belong to a highly correlated avalanche state. However, whether the plastic events …

Reaching the ideal glass in polymer spheres: Thermodynamics and vibrational density of states

X Monnier, J Colmenero, M Wolf, D Cangialosi - Physical review letters, 2021 - APS
The existence of an ideal glass and the resolution to the Kauzmann paradox is a long-
standing open question in materials science. To address this problem, we exploit the ability …

Atomistic structural mechanism for the glass transition: Entropic contribution

D Han, D Wei, J Yang, HL Li, MQ Jiang, YJ Wang… - Physical Review B, 2020 - APS
A popular Adam-Gibbs scenario has suggested that the excess entropy of glass and liquid
over crystal dominates the dynamical arrest at the glass transition with exclusive contribution …

Creating bulk ultrastable glasses by random particle bonding

M Ozawa, Y Iwashita, W Kob, F Zamponi - Nature Communications, 2023 - nature.com
A recent breakthrough in glass science has been the synthesis of ultrastable glasses via
physical vapor deposition techniques. These samples display enhanced thermodynamic …

Exploring the soft pinning effect in the dynamics and the structure–dynamics correlation in multicomponent supercooled liquids

E Anwar, P Patel, M Sharma… - The Journal of …, 2024 - pubs.aip.org
We study multicomponent liquids by increasing the mass of 15% of the particles in a binary
Kob–Andersen model. We find that the heavy particles have dual effects on the lighter …

Configurational entropy of polydisperse supercooled liquids

M Ozawa, G Parisi, L Berthier - The Journal of Chemical Physics, 2018 - pubs.aip.org
We propose a computational method to measure the configurational entropy in generic
polydisperse glass-formers. In particular, our method resolves issues related to the diverging …

Computer simulations of the glass transition and glassy materials

JL Barrat, L Berthier - Comptes …, 2023 - comptes-rendus.academie-sciences …
We provide an overview of the different types of computational techniques developed over
the years to study supercooled liquids, glassy materials and the physics of the glass …