Transition-Metal-Catalyzed, Coordination-Assisted Functionalization of Nonactivated C(sp3)–H Bonds

B Liu, AM Romine, CZ Rubel, KM Engle… - Chemical reviews, 2021 - ACS Publications
Transition-metal-catalyzed, coordination-assisted C (sp3)–H functionalization has
revolutionized synthetic planning over the past few decades as the use of these directing …

Bidentate directing groups: an efficient tool in C–H bond functionalization chemistry for the expedient construction of C–C bonds

S Rej, Y Ano, N Chatani - Chemical reviews, 2020 - ACS Publications
During the past decades, synthetic organic chemistry discovered that directing group
assisted C–H activation is a key tool for the expedient and siteselective construction of C–C …

Palladium-catalyzed transformations of alkyl C–H bonds

J He, M Wasa, KSL Chan, Q Shao, JQ Yu - Chemical Reviews, 2017 - ACS Publications
This Review summarizes the advancements in Pd-catalyzed C (sp3)–H activation via
various redox manifolds, including Pd (0)/Pd (II), Pd (II)/Pd (IV), and Pd (II)/Pd (0). While few …

Transition metal-catalyzed C–H bond functionalizations by the use of diverse directing groups

Z Chen, B Wang, J Zhang, W Yu, Z Liu… - Organic Chemistry …, 2015 - pubs.rsc.org
Transition metal-catalyzed direct functionalization of C–H bonds is one of the key emerging
strategies that is currently attracting tremendous attention with the aim to provide alternative …

Computational studies of carboxylate-assisted C–H activation and functionalization at group 8–10 transition metal centers

DL Davies, SA Macgregor, CL McMullin - Chemical reviews, 2017 - ACS Publications
Computational studies on carboxylate-assisted C–H activation and functionalization at
group 8–10 transition metal centers are reviewed. This Review is organized by metal and …

Overcoming the Limitations of γ-and δ-C–H Arylation of Amines through Ligand Development

YQ Chen, Z Wang, Y Wu, SR Wisniewski… - Journal of the …, 2018 - ACS Publications
L, X-Type transient directing groups (TDGs) based on a reversible imine linkage have
emerged as broadly useful tools for C–H activation of ketones and free amines. However …

Ligand-Enabled Pd(II)-Catalyzed β-Methylene C(sp3)–H Arylation of Free Aliphatic Acids

L Hu, G Meng, JQ Yu - Journal of the American Chemical Society, 2022 - ACS Publications
Ligand development has enabled rapid advances in Pd (II)-catalyzed β-methyl C (sp3)–H
activation of free carboxylic acids. However, there are only a handful of reports of free-acid …

Reusable directing groups [8-aminoquinoline, picolinamide, sulfoximine] in C (sp3)–H bond activation: present and future

RK Rit, MR Yadav, K Ghosh, AK Sahoo - Tetrahedron, 2015 - Elsevier
This report briefly discusses the reusable directing group assisted functionalization of
unactivated remote alkyl C–H bonds and their synthetic potential in organic chemistry. The …

On the Mechanism and Selectivity of Palladium-Catalyzed C(sp3)–H Arylation of Pyrrolidines and Piperidines at Unactivated C4 Positions: Discovery of an Improved …

D Antermite, AJP White, L Casarrubios, JA Bull - ACS Catalysis, 2023 - ACS Publications
Directed C–H functionalization is a powerful means to functionalize otherwise unreactive C–
H bonds, for which aminoquinoline amides provide a powerful and frequently used directing …

Palladium(II)‐Catalyzed Enantioselective Arylation of Unbiased Methylene C(sp3)−H Bonds Enabled by a 2‐Pyridinylisopropyl Auxiliary and Chiral Phosphoric Acids

SY Yan, YQ Han, QJ Yao, XL Nie… - Angewandte Chemie …, 2018 - Wiley Online Library
Enantioselective functionalizations of unbiased methylene C (sp3)− H bonds of linear
systems by metal insertion are intrinsically challenging and remain a largely unsolved …