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Direct methane oxidation by copper-and iron-dependent methane monooxygenases
Methane is a potent greenhouse gas that contributes significantly to climate change and is
primarily regulated in Nature by methanotrophic bacteria, which consume methane gas as …
primarily regulated in Nature by methanotrophic bacteria, which consume methane gas as …
Applications of halogen-atom transfer (XAT) for the generation of carbon radicals in synthetic photochemistry and photocatalysis
The halogen-atom transfer (XAT) is one of the most important and applied processes for the
generation of carbon radicals in synthetic chemistry. In this review, we summarize and …
generation of carbon radicals in synthetic chemistry. In this review, we summarize and …
Single atom catalysts for selective methane oxidation to oxygenates
Direct conversion of methane (CH4) to C1–2 liquid oxygenates is a captivating approach to
lock carbons in transportable value-added chemicals, while reducing global warming …
lock carbons in transportable value-added chemicals, while reducing global warming …
Oxidative addition of an alkyl halide to form a stable Cu (III) product
The step that cleaves the carbon-halogen bond in copper-catalyzed cross-coupling
reactions remains ill defined because of the multiple redox manifolds available to copper …
reactions remains ill defined because of the multiple redox manifolds available to copper …
Copper-mediated synthesis of drug-like bicyclopentanes
Multicomponent reactions are relied on in both academic and industrial synthetic organic
chemistry owing to their step-and atom-economy advantages over traditional synthetic …
chemistry owing to their step-and atom-economy advantages over traditional synthetic …
Creation from Confusion and Fusion in the Porphyrin World─ The Last Three Decades of N-Confused Porphyrinoid Chemistry
Confusion is a novel concept of isomerism in porphyrin chemistry, delivering a steady
stream of new chemistry since the discovery of N-confused porphyrin, a porphyrin mutant, in …
stream of new chemistry since the discovery of N-confused porphyrin, a porphyrin mutant, in …
Cobalt-Catalyzed Carbon–Heteroatom Transfer Enables Regioselective Tricomponent 1, 4-Carboamination
Tricomponent cobalt (salen)-catalyzed carbofunctionalization of unsaturated substrates by
radical–polar crossover has the potential to streamline access to broad classes of …
radical–polar crossover has the potential to streamline access to broad classes of …
Catalytically relevant organocopper (III) complexes formed through aryl-radical-enabled oxidative addition
Stepwise oxidative addition of copper (I) complexes to form copper (III) species via single
electron transfer (SET) events has been widely proposed in copper catalysis. However …
electron transfer (SET) events has been widely proposed in copper catalysis. However …
Cross-coupling by a noncanonical mechanism involving the addition of aryl halide to Cu (II)
Copper complexes are widely used in the synthesis of fine chemicals and materials to
catalyze couplings of heteroatom nucleophiles with aryl halides. We show that cross …
catalyze couplings of heteroatom nucleophiles with aryl halides. We show that cross …
Defect engineering of ceria nanocrystals for enhanced catalysis via a high-entropy oxide strategy
Introducing transition-metal components to ceria (CeO2) is important to tailor the surface
redox properties for a broad scope of applications. The emergence of high-entropy oxides …
redox properties for a broad scope of applications. The emergence of high-entropy oxides …