Transient directing ligands for selective metal-catalysed C–H activation

N Goswami, T Bhattacharya, D Maiti - Nature Reviews Chemistry, 2021‏ - nature.com
C–H activation is a 'simple-to-complex'transformation that nature has perfected over millions
of years of evolution. Transition-metal-catalysed C–H activation has emerged as an …

Transient Ligand‐Enabled Transition Metal‐Catalyzed C− H Functionalization

B Niu, K Yang, B Lawrence, H Ge - ChemSusChem, 2019‏ - Wiley Online Library
Transition metal‐catalyzed C− H bond functionalization is among the most efficient and
powerful strategies in synthetic organic chemistry to derivatize otherwise inert sites of …

Transient imines as 'next generation'directing groups for the catalytic functionalisation of C–H bonds in a single operation

S St John-Campbell, JA Bull - Organic & Biomolecular Chemistry, 2018‏ - pubs.rsc.org
C–H functionalisation promises a paradigm shift in synthetic planning. However, the
additional steps often required to install and remove directing groups currently detract from …

Transient directing groups in metal− organic cooperative catalysis

C Jacob, BUW Maes, G Evano - Chemistry–A European …, 2021‏ - Wiley Online Library
The direct functionalization of C− H bonds is among the most fundamental chemical
transformations in organic synthesis. However, when the innate reactivity of the substrate …

Combining transition metals and transient directing groups for C–H functionalizations

T Bhattacharya, S Pimparkar, D Maiti - RSC advances, 2018‏ - pubs.rsc.org
In the domain of synthetic chemistry, C–H bond activation has always remained in the
spotlight for researchers over the last few decades. Although different strategies have been …

Advances in development of C–H activation/functionalization using a catalytic directing group

OK Rasheed, B Sun - ChemistrySelect, 2018‏ - Wiley Online Library
The transition metal catalyzed direct site‐selective carbon–hydrogen functionalization is
ubiquitous in organic synthesis and has reached an impressive level of sophistication and …

Monodentate Transient Directing Group Assisted Ruthenium(II)-Catalyzed Direct ortho-C–H Imidation of Benzaldehydes for Diverse Synthesis of Quinazoline and …

Y Wu, N Liu, M Qi, H Qiao, X Lu, L Ma, Y Zhou… - Organic …, 2021‏ - ACS Publications
2-Fluoro-5-(trifluoromethyl) aniline was found to be a suitable monodentate transient
directing group (MonoTDG) to enable Ru (II)-catalyzed intermolecular direct ortho-C (sp2)–H …

Transition Metal-Catalyzed CH Activation via Imine-Based Transient Directing Group Strategy

Y Wu, B Shi - Chinese Journal of Organic Chemistry, 2020‏ - sioc-journal.cn
In the past decades, transition metal-catalyzed C—H activation has experienced
tremendous growth and revolutionized the field of organic synthesis. Several elegant …

Manganese-Catalyzed ortho-CH Amidation of Weakly Coordinating Aromatic Ketones

X Kong, B Xu - Organic Letters, 2018‏ - ACS Publications
An efficient manganese-catalyzed ortho-CH amidation of weakly coordinating aromatic
ketones using the readily available sulfonyl azide as the amination reagent is developed …

Cp*Co(III)‐Catalyzed o‐Amidation of Benzaldehydes with Dioxazolones Using Transient Directing Group Strategy

B Khan, V Dwivedi… - Advanced Synthesis & …, 2020‏ - Wiley Online Library
Transition metal‐catalyzed ortho‐selective C (sp2)− H amidation of weakly coordinating
aldehydes remains limited to precious metals such as Ir, Rh, Ru, etc. Herein, we put forward …