Molecular spins for quantum computation

A Gaita-Ariño, F Luis, S Hill, E Coronado - Nature chemistry, 2019 - nature.com
Spins in solids or in molecules possess discrete energy levels, and the associated quantum
states can be tuned and coherently manipulated by means of external electromagnetic …

Silicon quantum electronics

FA Zwanenburg, AS Dzurak, A Morello… - Reviews of modern …, 2013 - APS
This review describes recent groundbreaking results in Si, Si/SiGe, and dopant-based
quantum dots, and it highlights the remarkable advances in Si-based quantum physics that …

A single-atom electron spin qubit in silicon

JJ Pla, KY Tan, JP Dehollain, WH Lim, JJL Morton… - Nature, 2012 - nature.com
A single atom is the prototypical quantum system, and a natural candidate for a quantum bit,
or qubit—the elementary unit of a quantum computer. Atoms have been successfully used to …

Potential for spin-based information processing in a thin-film molecular semiconductor

M Warner, S Din, IS Tupitsyn, GW Morley… - Nature, 2013 - nature.com
Organic semiconductors are studied intensively for applications in electronics and optics,
and even spin-based information technology, or spintronics. Fundamental quantities in …

Quantum oscillations in a molecular magnet

S Bertaina, S Gambarelli, T Mitra, B Tsukerblat… - Nature, 2008 - nature.com
The term 'molecular magnet'generally refers to a molecular entity containing several
magnetic ions whose coupled spins generate a collective spin, S (ref.). Such complex multi …

Coherent two-dimensional terahertz magnetic resonance spectroscopy of collective spin waves

J Lu, X Li, HY Hwang, BK Ofori-Okai, T Kurihara… - Physical review …, 2017 - APS
We report a demonstration of two-dimensional (2D) terahertz (THz) magnetic resonance
spectroscopy using the magnetic fields of two time-delayed THz pulses. We apply the …

Spin-based quantum computers made by chemistry: hows and whys

PCE Stamp, A Gaita-Arino - Journal of Materials Chemistry, 2009 - pubs.rsc.org
This introductory review discusses the main problems facing the attempt to build quantum
information processing systems (like quantum computers) from spin-based qubits. We …

Electron spin decoherence in isotope-enriched silicon

WM Witzel, MS Carroll, A Morello, Ł Cywiński… - Physical review …, 2010 - APS
Silicon is promising for spin-based quantum computation because nuclear spins, a source of
magnetic noise, may be eliminated through isotopic enrichment. Long spin decoherence …

Endohedral Metallofullerene as Molecular High Spin Qubit: Diverse Rabi Cycles in Gd2@C79N

Z Hu, BW Dong, Z Liu, JJ Liu, J Su, C Yu… - Journal of the …, 2018 - ACS Publications
An anisotropic high-spin qubit with long coherence time could scale the quantum system up.
It has been proposed that Grover's algorithm can be implemented in such systems …

Toward molecular spin qubit devices: Integration of magnetic molecules into solid-state devices

AA Fursina, A Sinitskii - ACS Applied Electronic Materials, 2023 - ACS Publications
We review the progress made in integrating magnetic molecules containing transition metal
ions into nanoelectronic solid-state devices and using them as molecular spin qubits …