Best‐practice DFT protocols for basic molecular computational chemistry

M Bursch, JM Mewes, A Hansen… - Angewandte Chemie …, 2022 - Wiley Online Library
Nowadays, many chemical investigations are supported by routine calculations of molecular
structures, reaction energies, barrier heights, and spectroscopic properties. The lion's share …

Machine learning force fields

OT Unke, S Chmiela, HE Sauceda… - Chemical …, 2021 - ACS Publications
In recent years, the use of machine learning (ML) in computational chemistry has enabled
numerous advances previously out of reach due to the computational complexity of …

Independent gradient model based on Hirshfeld partition: A new method for visual study of interactions in chemical systems

T Lu, Q Chen - Journal of computational chemistry, 2022 - Wiley Online Library
The powerful independent gradient model (IGM) method has been increasingly popular in
visual analysis of intramolecular and intermolecular interactions in recent years. However …

In situ Raman spectroscopy reveals the structure and dissociation of interfacial water

YH Wang, S Zheng, WM Yang, RY Zhou, QF He… - Nature, 2021 - nature.com
Understanding the structure and dynamic process of water at the solid–liquid interface is an
extremely important topic in surface science, energy science and catalysis,–. As model …

Rational design of Lewis base molecules for stable and efficient inverted perovskite solar cells

C Li, X Wang, E Bi, F Jiang, SM Park, Y Li, L Chen… - Science, 2023 - science.org
Lewis base molecules that bind undercoordinated lead atoms at interfaces and grain
boundaries (GBs) are known to enhance the durability of metal halide perovskite solar cells …

Epitaxial growth of wafer-scale molybdenum disulfide semiconductor single crystals on sapphire

T Li, W Guo, L Ma, W Li, Z Yu, Z Han, S Gao… - Nature …, 2021 - nature.com
Abstract Two-dimensional (2D) semiconductors, in particular transition metal
dichalcogenides (TMDCs), have attracted great interest in extending Moore's law beyond …

Stability-limiting heterointerfaces of perovskite photovoltaics

S Tan, T Huang, I Yavuz, R Wang, TW Yoon, M Xu… - Nature, 2022 - nature.com
Optoelectronic devices consist of heterointerfaces formed between dissimilar
semiconducting materials. The relative energy-level alignment between contacting …

High carbon utilization in CO2 reduction to multi-carbon products in acidic media

Y ** of perovskite semiconductors and passivation of their grain boundaries remain
challenging but essential for advancing high-efficiency perovskite solar cells. Particularly, it …