Data generation for machine learning interatomic potentials and beyond

M Kulichenko, B Nebgen, N Lubbers, JS Smith… - Chemical …, 2024 - ACS Publications
The field of data-driven chemistry is undergoing an evolution, driven by innovations in
machine learning models for predicting molecular properties and behavior. Recent strides in …

Bayesian optimization for chemical reactions

J Guo, B Ranković, P Schwaller - Chimia, 2023 - chimia.ch
Reaction optimization is challenging and traditionally delegated to domain experts who
iteratively propose increasingly optimal experiments. Problematically, the reaction …

Accelerating explicit solvent models of heterogeneous catalysts with machine learning interatomic potentials

BWJ Chen, X Zhang, J Zhang - Chemical Science, 2023 - pubs.rsc.org
Realistically modelling how solvents affect catalytic reactions is a longstanding challenge
due to its prohibitive computational cost. Typically, an explicit atomistic treatment of the …

3DReact: Geometric Deep Learning for Chemical Reactions

P van Gerwen, KR Briling, C Bunne… - Journal of chemical …, 2024 - ACS Publications
Geometric deep learning models, which incorporate the relevant molecular symmetries
within the neural network architecture, have considerably improved the accuracy and data …

Comment on 'physics-based representations for machine learning properties of chemical reactions'

KA Spiekermann, T Stuyver, L Pattanaik… - Machine Learning …, 2023 - iopscience.iop.org
In a recent article in this journal, van Gerwen et al (2022 Mach. Learn.: Sci. Technol. 3
045005) presented a kernel ridge regression model to predict reaction barrier heights. Here …

[HTML][HTML] Asparagus: A toolkit for autonomous, user-guided construction of machine-learned potential energy surfaces

K Töpfer, LI Vazquez-Salazar, M Meuwly - Computer Physics …, 2025 - Elsevier
With the establishment of machine learning (ML) techniques in the scientific community, the
construction of ML potential energy surfaces (ML-PES) has become a standard process in …

Bayesian optimisation for additive screening and yield improvements–beyond one-hot encoding

B Ranković, RR Griffiths, HB Moss, P Schwaller - Digital Discovery, 2024 - pubs.rsc.org
Reaction additives are critical in dictating the outcomes of chemical processes making their
effective screening vital for research. Conventional high-throughput experimentation tools …

Partial density of states representation for accurate deep neural network predictions of x-ray spectra

C Middleton, BFE Curchod, TJ Penfold - Physical Chemistry Chemical …, 2024 - pubs.rsc.org
The performance of a machine learning (ML) algorithm for chemistry is highly contingent
upon the architect's choice of input representation. This work introduces the partial density of …

Structure-free Mendeleev encodings of material compounds for machine learning

Z Zhuang, AS Barnard - Chemistry of Materials, 2023 - ACS Publications
Machine learning is a powerful tool to predict the properties of materials for a variety of
applications. However, generating data sets of carefully characterized materials can be time …

Genetic algorithms for the discovery of homogeneous catalysts

S Gallarati, P Van Gerwen, AA Schoepfer, R Laplaza… - Chimia, 2023 - chimia.ch
In this account, we discuss the use of genetic algorithms in the inverse design process of
homogeneous catalysts for chemical transformations. We describe the main components of …