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Few-optical-cycle pulses tunable from the visible to the mid-infrared by optical parametric amplifiers
Ultrafast optical parametric amplifiers (OPAs) can provide, under suitable conditions, ultra-
broad gain bandwidths and can thus be used as effective tools for the generation of widely …
broad gain bandwidths and can thus be used as effective tools for the generation of widely …
Few‐optical‐cycle light pulses with passive carrier‐envelope phase stabilization
One of the most advanced frontiers of ultrafast optics is the control of carrier‐envelope phase
(CEP) ϕ of light pulses, which enables the generation of optical waveforms with …
(CEP) ϕ of light pulses, which enables the generation of optical waveforms with …
Design criteria for ultrafast optical parametric amplifiers
Optical parametric amplifiers (OPAs) exploit second-order nonlinearity to transfer energy
from a fixed frequency pump pulse to a variable frequency signal pulse, and represent an …
from a fixed frequency pump pulse to a variable frequency signal pulse, and represent an …
The role of spin in the kinetic control of recombination in organic photovoltaics
In biological complexes, cascade structures promote the spatial separation of
photogenerated electrons and holes, preventing their recombination. In contrast, the …
photogenerated electrons and holes, preventing their recombination. In contrast, the …
Vibronically coherent ultrafast triplet-pair formation and subsequent thermally activated dissociation control efficient endothermic singlet fission
Singlet exciton fission (SF), the conversion of one spin-singlet exciton (S1) into two spin-
triplet excitons (T1), could provide a means to overcome the Shockley–Queisser limit in …
triplet excitons (T1), could provide a means to overcome the Shockley–Queisser limit in …
Identification of a triplet pair intermediate in singlet exciton fission in solution
Singlet exciton fission is the spin-conserving transformation of one spin-singlet exciton into
two spin-triplet excitons. This exciton multiplication mechanism offers an attractive route to …
two spin-triplet excitons. This exciton multiplication mechanism offers an attractive route to …
The nature of singlet exciton fission in carotenoid aggregates
Singlet exciton fission allows the fast and efficient generation of two spin triplet states from
one photoexcited singlet. It has the potential to improve organic photovoltaics, enabling …
one photoexcited singlet. It has the potential to improve organic photovoltaics, enabling …
Activated singlet exciton fission in a semiconducting polymer
Singlet exciton fission is a spin-allowed process to generate two triplet excitons from a single
absorbed photon. This phenomenon offers great potential in organic photovoltaics, but the …
absorbed photon. This phenomenon offers great potential in organic photovoltaics, but the …
High-time-resolution pump-probe system with broadband detection for the study of time-domain vibrational dynamics
We present an ultrafast transient absorption spectroscopy system in the visible combining
high-sensitivity broadband detection with extreme temporal resolution. The instrument is …
high-sensitivity broadband detection with extreme temporal resolution. The instrument is …
Quantitative bimolecular recombination in organic photovoltaics through triplet exciton formation
The nanoscale morphology and high charge densities in organic photovoltaics (OPVs) lead
to a high rate of bimolecular encounters between spin-uncorrelated electrons and holes …
to a high rate of bimolecular encounters between spin-uncorrelated electrons and holes …