Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Enrichment of reactants and intermediates for electrocatalytic CO 2 reduction

PP Yang, MR Gao - Chemical Society Reviews, 2023 - pubs.rsc.org
The electrocatalytic carbon dioxide reduction reaction (CO2RR) presents a sustainable
route to convert renewable electricity to value-added fuels and feedstocks in the form of …

Cationic-group-functionalized electrocatalysts enable stable acidic CO2 electrolysis

M Fan, JE Huang, RK Miao, Y Mao, P Ou, F Li, XY Li… - Nature Catalysis, 2023 - nature.com
Acidic electrochemical CO2 reduction (CO2R) addresses CO2 loss and thus mitigates the
energy penalties associated with CO2 recovery; however, acidic CO2R suffers low …

CO2 electroreduction to multicarbon products in strongly acidic electrolyte via synergistically modulating the local microenvironment

Z Ma, Z Yang, W Lai, Q Wang, Y Qiao, H Tao… - Nature …, 2022 - nature.com
Electrochemical CO2 reduction to multicarbon products faces challenges of unsatisfactory
selectivity, productivity, and long-term stability. Herein, we demonstrate CO2 …

Surface hydroxide promotes CO2 electrolysis to ethylene in acidic conditions

Y Cao, Z Chen, P Li, A Ozden, P Ou, W Ni… - Nature …, 2023 - nature.com
Performing CO2 reduction in acidic conditions enables high single-pass CO2 conversion
efficiency. However, a faster kinetics of the hydrogen evolution reaction compared to CO2 …

Gas diffusion electrodes and membranes for CO2 reduction electrolysers

EW Lees, BAW Mowbray, FGL Parlane… - Nature Reviews …, 2022 - nature.com
The CO2 reduction reaction (CO2RR) is a potential means of using renewable electricity to
synthesize commodity chemicals and fuels. The CO2RR can be performed at industrially …

Membrane Electrode Assembly for Electrocatalytic CO2 Reduction: Principle and Application

Z Zhang, X Huang, Z Chen, J Zhu… - Angewandte …, 2023 - Wiley Online Library
Electrocatalytic CO2 reduction reaction (CO2RR) in membrane electrode assembly (MEA)
systems is a promising technology. Gaseous CO2 can be directly transported to the cathode …

Electrochemical reduction of carbon dioxide to multicarbon (C 2+) products: challenges and perspectives

B Chang, H Pang, F Raziq, S Wang… - Energy & …, 2023 - pubs.rsc.org
Electrocatalytic CO2 reduction has been developed as a promising and attractive strategy to
achieve carbon neutrality for sustainable chemical production. Among various reduction …

Close to 90% Single-Pass Conversion Efficiency for CO2 Electroreduction in an Acid-Fed Membrane Electrode Assembly

B Pan, J Fan, J Zhang, Y Luo, C Shen, C Wang… - ACS Energy …, 2022 - ACS Publications
The formation of (bi) carbonates is a pressing issue for CO2 electroreduction in neutral or
alkaline solutions. It adversely causes low single-pass conversion efficiency as a result of …

CO2 electrolysis to multicarbon products in strong acid

JE Huang, F Li, A Ozden, A Sedighian Rasouli… - Science, 2021 - science.org
Carbon dioxide electroreduction (CO2R) is being actively studied as a promising route to
convert carbon emissions to valuable chemicals and fuels. However, the fraction of input …