Laser ablation plasmas and spectroscopy for nuclear applications
EH Kwapis, J Borrero, KS Latty, HB Andrews… - Applied …, 2024 - opg.optica.org
The development of measurement methodologies to detect and monitor nuclear-relevant
materials remains a consistent and significant interest across the nuclear energy …
materials remains a consistent and significant interest across the nuclear energy …
Optical spectroscopy and modeling of uranium gas-phase oxidation: Progress and perspectives
Studies related to U gas-phase oxidation through plasma-and thermo-chemistry are
important for many fields, including environmental monitoring, forensic analysis, debris …
important for many fields, including environmental monitoring, forensic analysis, debris …
Review on recent advances in analytical applications of molecular emission and modelling
The review mainly deals with two topics that became important in applications of laser-
induced breakdown spectroscopy (LIBS) in recent years: the emission of halogen-and rare …
induced breakdown spectroscopy (LIBS) in recent years: the emission of halogen-and rare …
Laser ablation spectrometry for studies of uranium plasmas, reactor monitoring, and spent fuel safety
Nuclear security is one of the defining challenges of our time. Nuclear threats range from
deliberate dispersal of radioactive material to contaminate the vital infrastructure to diversion …
deliberate dispersal of radioactive material to contaminate the vital infrastructure to diversion …
Spectroscopic signatures and oxidation characteristics of nanosecond laser-induced cerium plasmas
EH Kwapis, E Villa-Aleman, KC Hartig - Spectrochimica Acta Part B: Atomic …, 2023 - Elsevier
Improving technologies related to the wide area environmental sampling of nuclear
materials supports the nuclear nonproliferation mission of preventing the proliferation of …
materials supports the nuclear nonproliferation mission of preventing the proliferation of …
Physical conditions for UO formation in laser-produced uranium plumes
We investigate the oxidation of uranium (U) species, the physical conditions leading to
uranium monoxide (UO) formation and the interplay between plume hydrodynamics and …
uranium monoxide (UO) formation and the interplay between plume hydrodynamics and …
The role of ambient gas confinement, plasma chemistry, and focusing conditions on emission features of femtosecond laser-produced plasmas
Ultrafast laser ablation coupled with optical emission spectroscopy is currently under
development for standoff detection of elements and their isotopes for a wide range of …
development for standoff detection of elements and their isotopes for a wide range of …
The effect of oxygen concentration on the speciation of laser ablated uranium
MA Burton, AW Auner, JC Crowhurst, PS Boone… - Scientific Reports, 2022 - nature.com
In order to model the fate and transport of particles following a nuclear explosion, there must
first be an understanding of individual physical and chemical processes that affect particle …
first be an understanding of individual physical and chemical processes that affect particle …
Unraveling spatio-temporal chemistry evolution in laser ablation plumes and its relation to initial plasma conditions
The chemistry evolution in a laser ablation plume depends strongly on its initial physical
conditions. In this article, we investigate the impact of plasma generation conditions on the …
conditions. In this article, we investigate the impact of plasma generation conditions on the …
Time-resolved imaging of atoms and molecules in laser-produced uranium plasmas
Gas-phase oxidation of uranium (U), plume chemistry, and the corresponding impact on
optical emission features of the U plasma are investigated. Plasmas were produced via …
optical emission features of the U plasma are investigated. Plasmas were produced via …