Generation, manipulation and characterization of molecules by atomic force microscopy
Using atomic manipulation, one can dissociate, form and rearrange bonds, as well as alter
the conformation or charge state of molecules. The molecular structures of reactants …
the conformation or charge state of molecules. The molecular structures of reactants …
On-surface generation and imaging of arynes by atomic force microscopy
Reactive intermediates are involved in many chemical transformations. However, their
characterization is a great challenge because of their short lifetimes and high reactivities …
characterization is a great challenge because of their short lifetimes and high reactivities …
Self‐Template‐Directed Metal–Organic Frameworks Network and the Derived Honeycomb‐Like Carbon Flakes via Confinement Pyrolysis
Metal–organic frameworks (MOFs) have become a research hotspot since they have been
explored as convenient precursors for preparing various multifunctional nanomaterials …
explored as convenient precursors for preparing various multifunctional nanomaterials …
Generation and Characterization of a meta-Aryne on Cu and NaCl Surfaces
We describe the generation of a meta-aryne at low temperature (T= 5 K) using atomic
manipulation on Cu (111) and on bilayer NaCl on Cu (111). We observe different voltage …
manipulation on Cu (111) and on bilayer NaCl on Cu (111). We observe different voltage …
Atomically resolved real-space imaging of hot electron dynamics
The dynamics of hot electrons are central to understanding the properties of many electronic
devices. But their ultra-short lifetime, typically 100 fs or less, and correspondingly short …
devices. But their ultra-short lifetime, typically 100 fs or less, and correspondingly short …
High-voltage-assisted mechanical stabilization of single-molecule junctions
Resonant tunneling is an efficient mechanism for charge transport through nanoscale
conductance junctions due to the relatively high currents involved. However, continuous …
conductance junctions due to the relatively high currents involved. However, continuous …
Non-adiabatic effects of nuclear motion in quantum transport of electrons: A self-consistent Keldysh–Langevin study
VF Kershaw, DS Kosov - The Journal of Chemical Physics, 2020 - pubs.aip.org
The molecular junction geometry is modeled in terms of nuclear degrees of freedom that are
embedded in a stochastic quantum environment of non-equilibrium electrons. The time …
embedded in a stochastic quantum environment of non-equilibrium electrons. The time …
Direct and delayed dynamics in electron-induced surface reaction
The electron-induced reaction of physisorbed vinyl bromide (ViBr) and allyl bromide (AllBr)
on Cu (110) at 4.6 K was studied experimentally by scanning tunneling microscopy and …
on Cu (110) at 4.6 K was studied experimentally by scanning tunneling microscopy and …
Desorption induced by low energy charge carriers on Si (111)‐7× 7: First principles molecular dynamics for benzene derivates
We use clusters for the modeling of local ion resonances caused by low energy charge
carriers in STM‐induced desorption of benzene derivates from Si (111)‐7× 7. We perform …
carriers in STM‐induced desorption of benzene derivates from Si (111)‐7× 7. We perform …
Clocking surface reaction by in-plane product rotation
Electron-induced reaction of physisorbed meta-diiodobenzene (mDIB) on Cu (110) at 4.6 K
was studied by Scanning Tunneling Microscopy and molecular dynamics theory. Single …
was studied by Scanning Tunneling Microscopy and molecular dynamics theory. Single …