Aqueous iron (IV)–oxo complex: an emerging powerful reactive oxidant formed by iron (II)-based advanced oxidation processes for oxidative water treatment

Z Wang, W Qiu, S Pang, Q Guo, C Guan… - … Science & Technology, 2022 - ACS Publications
High-valent iron (IV)–oxo complexes are of great significance as reactive intermediates
implicated in diverse chemical and biological systems. The aqueous iron (IV)–oxo complex …

Dioxygen activation at mononuclear nonheme iron active sites: enzymes, models, and intermediates

M Costas, MP Mehn, MP Jensen, L Que - Chemical reviews, 2004 - ACS Publications
There have been significant advances in our understanding of mononuclear nonheme iron
oxygenases since our 1996 Chemical Reviews article, 1 promoted in large part by the many …

α-Fe2O3 as a versatile and efficient oxygen atom transfer catalyst in combination with H2O as the oxygen source

Y Zhao, C Deng, D Tang, L Ding, Y Zhang, H Sheng… - Nature Catalysis, 2021 - nature.com
Abstract Haematite (α-Fe2O3) has been extensively investigated as a photoanode in
photoelectrochemical water oxidation, but the product O2 has a low economic value. Here …

Prediction of molecular properties and molecular spectroscopy with density functional theory: From fundamental theory to exchange-coupling

F Neese - Coordination Chemistry Reviews, 2009 - Elsevier
This review provides a detailed account of density functional theory (DFT) and its application
to the calculation of molecular properties of inorganic compounds. After introducing some …

High-valent iron (IV)–oxo complexes of heme and non-heme ligands in oxygenation reactions

W Nam - Accounts of chemical research, 2007 - ACS Publications
High-valent iron (IV)–oxo species have been implicated as the key reactive intermediates in
the catalytic cycles of dioxygen activation by heme and non-heme iron enzymes. Our …

Fe (II)/α-ketoglutarate-dependent hydroxylases and related enzymes

RP Hausinger - Critical reviews in biochemistry and molecular …, 2004 - Taylor & Francis
Fe (II)/α-ketoglutarate (αKG)-dependent hydroxylases catalyze an amazing diversity of
reactions that result in protein side-chain modifications, repair of alkylated DNA/RNA …

Efficient water oxidation catalysts based on readily available iron coordination complexes

JL Fillol, Z Codolà, I Garcia-Bosch, L Gómez, JJ Pla… - Nature …, 2011 - nature.com
Water oxidation catalysis constitutes the bottleneck for the development of energy-
conversion schemes based on sunlight. To date, state-of-the-art homogeneous water …

Non-heme Fe (IV)–oxo intermediates

C Krebs, D Galonic Fujimori, CT Walsh… - Accounts of chemical …, 2007 - ACS Publications
High-valent non-heme iron–oxo intermediates have been proposed for decades as the key
intermediates in numerous biological oxidation reactions. In the past three years, the first …

Recognition of surface oxygen intermediates on NiFe oxyhydroxide oxygen-evolving catalysts by homogeneous oxidation reactivity

Y Hao, Y Li, J Wu, L Meng, J Wang, C Jia… - Journal of the …, 2021 - ACS Publications
NiFe oxyhydroxide is one of the most promising oxygen evolution reaction (OER) catalysts
for renewable hydrogen production, and deciphering the identity and reactivity of the oxygen …

Reactive high-spin iron (IV)-oxo sites through dioxygen activation in a metal–organic framework

K Hou, J Börgel, HZH Jiang, DJ SantaLucia, H Kwon… - Science, 2023 - science.org
In nature, nonheme iron enzymes use dioxygen to generate high-spin iron (IV)= O species
for a variety of oxygenation reactions. Although synthetic chemists have long sought to …